Assembly of luminescent Ag(I) coordination architectures adjusted by modification of pyrimidine-based thioether ligands

被引：34

作者：

Han, L ^{[1
]}

Wu, BL ^{[1
]}

Xu, YQ ^{[1
]}

Wu, MY ^{[1
]}

Gong, YQ ^{[1
]}

Lou, BY ^{[1
]}

Chen, BQ ^{[1
]}

Hong, MC ^{[1
]}

机构：

[1] Chinese Acad Sci, Fujian Inst Res Struct Matter, State Key Lab Struct Chem, Fuzhou 350002, Peoples R China

来源：

INORGANICA CHIMICA ACTA | 2005年 / 358卷 / 06期

基金：

中国国家自然科学基金;

关键词：

silver complexes; thioether ligands; coordination architecture; self-assembly; ligand modification;

D O I：

10.1016/j.ica.2004.12.023

中图分类号：

O61 [无机化学];

学科分类号：

070301 ; 081704 ;

摘要：

Two new structurally related pyrimidine-based thioether ligands, angular ditopic ligand 1,3-bis(2-pyrimidinylthiomethyl)benzene (L-2) and linear ditopic ligand 1,4-bis(2-pyrimidinylthiomethyl)benzene (L-3), have been designed and prepared. Reaction of two shaped-specific ligands with different silver(I) salts affords three novel luminescent coordination architectures: discrete metallomacrocycle [Ag-4(L-2)(2)(NO3)(4)]center dot 2MeOH (3), 1D chain {[Ag2L3 (NO3)(2)]center dot 2CCl(3)}(n) (4) and 2D wire netlike structure {[AgL3 (DMF)]-ClO4 center dot 0.25H(2)O}n (5). The results show that the nature of organic ligands, geometric requirement of metal atoms and counter anions have great influence on the structures of metal-organic frameworks. (c) 2005 Elsevier B.V. All rights reserved.

引用

页码：2005 / 2013

页数：9

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