Assembly of luminescent Ag(I) coordination architectures adjusted by modification of pyrimidine-based thioether ligands

被引：34
|
作者：
Han, L [1 ]
Wu, BL [1 ]
Xu, YQ [1 ]
Wu, MY [1 ]
Gong, YQ [1 ]
Lou, BY [1 ]
Chen, BQ [1 ]
Hong, MC [1 ]
机构：
[1] Chinese Acad Sci, Fujian Inst Res Struct Matter, State Key Lab Struct Chem, Fuzhou 350002, Peoples R China
来源：
INORGANICA CHIMICA ACTA | 2005年 / 358卷 / 06期
基金：
中国国家自然科学基金;
关键词：
silver complexes; thioether ligands; coordination architecture; self-assembly; ligand modification;
D O I：
10.1016/j.ica.2004.12.023
中图分类号：
O61 [无机化学];
学科分类号：
070301 ; 081704 ;
摘要：
Two new structurally related pyrimidine-based thioether ligands, angular ditopic ligand 1,3-bis(2-pyrimidinylthiomethyl)benzene (L-2) and linear ditopic ligand 1,4-bis(2-pyrimidinylthiomethyl)benzene (L-3), have been designed and prepared. Reaction of two shaped-specific ligands with different silver(I) salts affords three novel luminescent coordination architectures: discrete metallomacrocycle [Ag-4(L-2)(2)(NO3)(4)]center dot 2MeOH (3), 1D chain {[Ag2L3 (NO3)(2)]center dot 2CCl(3)}(n) (4) and 2D wire netlike structure {[AgL3 (DMF)]-ClO4 center dot 0.25H(2)O}n (5). The results show that the nature of organic ligands, geometric requirement of metal atoms and counter anions have great influence on the structures of metal-organic frameworks. (c) 2005 Elsevier B.V. All rights reserved.
引用
收藏
页码：2005 / 2013
页数：9
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