Bis-, tris-, and tetrakis-N-(2-nitroxyethyl) derivatives of 1,1′-[methylenebis(oxy)]bis(triaz-1-ene 2-oxides)

被引：10

作者：

Smirnov, G. A. ^{[1
]}

Gordeev, P. B. ^{[1
]}

Nikitin, S. V. ^{[1
]}

Pokhvisneva, G. V. ^{[1
]}

Ternikova, T. V. ^{[1
]}

Chistokhvalov, I. M. ^{[2
]}

Luk'yanov, O. A. ^{[1
]}

机构：

[1] Russian Acad Sci, ND Zelinsky Inst Organ Chem, 47 Leninsky Prosp, Moscow 119991, Russia

[2] D Mendeleev Univ Chem Technol Russia, 9 Miusskaya Pl, Moscow 125047, Russia

来源：

RUSSIAN CHEMICAL BULLETIN | 2018年 / 67卷 / 09期

基金：

俄罗斯科学基金会;

关键词：

NO donors; 1,1 '-[methylenebis(oxy)]bis(triaz-1-ene 2-oxides); 2-bromoethyl derivatives; 2-hydroxyethyl derivatives; 2-nitroxyethyl derivatives; nitrates; alkylation; nitration; nucleophilic substitution; hydrolysis; METHYLENE-BIS(1-OXY-3,3-DIALKYL-1-TRIAZENE 2-OXIDES); OXIDE; SYSTEMS; ACID;

D O I：

10.1007/s11172-018-2274-5

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Synthesis of new potential NO donors in living organisms, 1,1'-[methylenebis(oxy)]bis(triaz-1-ene 2-oxides) bearing from two to four 2-nitroxyethyl groups at the nitrogen atoms was accomplished. The developed synthetic approaches involves either nucleophilic substitution of the bromine atoms of the corresponding N-2-bromoethyl derivatives of 1,1'-[methylenebis(oxy)]-bis(triaz-1-ene 2-oxides) or nitration of its 2-hydroxyethyl analogs. Some of the synthesized compounds are of interest as promising energetic materials.

引用

页码：1662 / 1670

页数：9

共 50 条

[1] Bis-, tris-, and tetrakis-N-(2-nitroxyethyl) derivatives of 1,1’-[methylenebis(oxy)]bis(triaz-1-ene 2-oxides)
G. A. Smirnov
P. B. Gordeev
S. V. Nikitin
G. V. Pokhvisneva
T. V. Ternikova
I. M. Chistokhvalov
O. A. Luk’yanov
Russian Chemical Bulletin, 2018, 67 : 1662 - 1670
[2] N--Nitroxyethyl derivatives of 1,1'-[methylenebis(oxy)]bis(triaz-1-ene 2-oxides)
Nikitin, S. V.
Pokhvisneva, G. V.
Ternikova, T. V.
Gordeev, P. B.
Chistokhvalov, I. M.
Smirnov, G. A.
Luk'yanov, O. A.
RUSSIAN CHEMICAL BULLETIN, 2018, 67 (08) : 1445 - 1451
[3] N-β-Nitroxyethyl derivatives of 1,1’-[methylenebis(oxy)]bis(triaz-1-ene 2-oxides)
S. V. Nikitin
G. V. Pokhvisneva
T. V. Ternikova
P. B. Gordeev
I. M. Chistokhvalov
G. A. Smirnov
O. A. Luk’yanov
Russian Chemical Bulletin, 2018, 67 : 1445 - 1451
[4] 3,3-Bis(2-nitroxyethyl) derivatives of 1,1′-[methylenebis(oxy)]bis(triaz-1-ene 2-oxides) as a new type of NO donors
Pokhvisneva, G. V.
Gordeev, P. B.
Nikitin, S. V.
Smirnov, G. A.
Ternikova, T. V.
Luk'yanov, O. A.
RUSSIAN CHEMICAL BULLETIN, 2018, 67 (09) : 1655 - 1661
[5] 3,3-Bis(2-nitroxyethyl) derivatives of 1,1′-[methylenebis(oxy)]bis(triaz-1-ene 2-oxides) as a new type of NO donors
G. V. Pokhvisneva
P. B. Gordeev
S. V. Nikitin
G. A. Smirnov
T. V. Ternikova
O. A. Luk’yanov
Russian Chemical Bulletin, 2018, 67 : 1655 - 1661
[6] Synthesis of 1,1'-[methylenebis(oxy)]-bis[3-alkyl-3-(2-hydroxyethyl)triaz-1-ene 2-oxides]
Pokhvisneva, G. V.
Ternikova, T. V.
Smirnov, G. A.
Gordeev, P. B.
Nikitin, S. V.
Luk'yanov, O. A.
RUSSIAN CHEMICAL BULLETIN, 2016, 65 (11) : 2650 - 2657
[7] Synthesis of 1,1´-[methylenebis(oxy)]bis[3-alkyl-3-(2-haloethyl)triaz-1-ene 2-oxides]
G. V. Pokhvisneva
T. V. Ternikova
G. A. Smirnov
P. B. Gordeev
S. V. Nikitin
O. A. Luk´yanov
Russian Chemical Bulletin, 2017, 66 : 1234 - 1239
[8] Synthesis of 1,1’-[methylenebis(oxy)]-bis[3-alkyl-3-(2-hydroxyethyl)triaz-1-ene 2-oxides]
G. V. Pokhvisneva
T. V. Ternikova
G. A. Smirnov
P. B. Gordeev
S. V. Nikitin
O. A. Luk’yanov
Russian Chemical Bulletin, 2016, 65 : 2650 - 2657
[9] Synthesis of 1,1A′-[methylenebis(oxy)]bis[3-alkyl-3-(2-haloethyl)triaz-1-ene 2-oxides]
Pokhvisneva, G. V.
Ternikova, T. V.
Smirnov, G. A.
Gordeev, P. B.
Nikitin, S. V.
Luk 'yanov, O. A.
RUSSIAN CHEMICAL BULLETIN, 2017, 66 (07) : 1234 - 1239
[10] Synthesis of 3,3-bis(2-haloethyl) and 3,3,3′-tris(2-haloethyl) derivatives of 1,1′-[methylenebis(oxy)]bis(triaz-1-ene 2-oxides)
T. V. Ternikova
G. V. Pokhvisneva
G. A. Smirnov
P. B. Gordeev
S. V. Nikitin
O. A. Luk’yanov
Russian Chemical Bulletin, 2017, 66 : 2103 - 2109

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