Determination of actinide and fission-product isotopes in very-high-burnup spent nuclear fuel

被引：0
|
作者：
V. S. Sullivan
D. L. Bowers
M. A. Clark
D. G. Graczyk
Y. Tsai
W. E. Streets
M. H. Vander Pol
M. C. Billone
机构：
[1] Argonne National Laboratory,Chemical Engineering Division
[2] Argonne National Laboratory,Energy Technology Division
来源：
Journal of Radioanalytical and Nuclear Chemistry | 2008年 / 277卷
关键词：
Plutonium; Thermal Ionization Mass Spectrometry; Nuclear Regulatory Commission; Chemical Engineer Division; Separate Rare Earth;
D O I：
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中图分类号：
学科分类号：
摘要：
A work plan was desired that would produce data for a wide array of actinide and fission-product isotopes with reasonably good accuracy and relatively low cost. An analysis scheme involving a fairly small number of separations, dilutions, and measurement methods was used to generate information on 74 isotopes in two spent-fuel samples of >70 GWd/MTU burnup. Some of the measured isotopes are of high interest for burnup-credit evaluations and had not been reported previously for high-burnup fuels.
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页码：59 / 64
页数：5
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