Determination of actinide and fission-product isotopes in very-high-burnup spent nuclear fuel

被引：9
|
作者：
Sullivan, V. S. [1 ]
Bowers, D. L. [1 ]
Clark, M. A. [1 ]
Graczyk, D. G. [1 ]
Tsai, Y. [1 ]
Streets, W. E. [1 ]
Pol, M. H. Vander [1 ]
Billone, M. C. [2 ]
机构：
[1] Argonne Natl Lab, Div Chem Engn, Argonne, IL 60439 USA
[2] Argonne Natl Lab, Div Energy Technol, Argonne, IL 60439 USA
来源：
JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY | 2008年 / 277卷 / 01期
关键词：
Plutonium; Thermal Ionization Mass Spectrometry; Nuclear Regulatory Commission; Chemical Engineer Division; Separate Rare Earth;
D O I：
10.1007/s10967-008-0709-4
中图分类号：
O65 [分析化学];
学科分类号：
070302 ; 081704 ;
摘要：
A work plan was desired that would produce data for a wide array of actinide and fission-product isotopes with reasonably good accuracy and relatively low cost. An analysis scheme involving a fairly small number of separations, dilutions, and measurement methods was used to generate information on 74 isotopes in two spent-fuel samples of > 70 GWd/MTU burnup. Some of the measured isotopes are of high interest for burnup-credit evaluations and had not been reported previously for high-burnup fuels.
引用
收藏
页码：59 / 64
页数：6
相关论文
共 50 条
  • [1] Determination of actinide and fission-product isotopes in very-high-burnup spent nuclear fuel
    V. S. Sullivan
    D. L. Bowers
    M. A. Clark
    D. G. Graczyk
    Y. Tsai
    W. E. Streets
    M. H. Vander Pol
    M. C. Billone
    [J]. Journal of Radioanalytical and Nuclear Chemistry, 2008, 277 : 59 - 64
  • [2] Determination of actinide and fission-product isotopes in very-high-burnup spent nuclear fuel.
    Bowers, DL
    Vander Pol, MH
    Clark, MA
    Graczyk, DG
    Streets, WE
    Tsai, YF
    Billone, MC
    [J]. ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 2004, 227 : U83 - U83
  • [3] FISSION-PRODUCT BEHAVIOR IN PHENIX FUEL-PINS AT HIGH BURNUP
    TOURASSE, M
    BOIDRON, M
    PASQUET, B
    [J]. JOURNAL OF NUCLEAR MATERIALS, 1992, 188 : 49 - 57
  • [4] FUEL BURNUP DETERMINATION BASED ON THE MEASUREMENT OF A SHORT-LIVED FISSION-PRODUCT
    WANG, TK
    SHIAO, LC
    TSENG, CL
    [J]. NUCLEAR TECHNOLOGY, 1990, 91 (03) : 413 - 418
  • [5] DETERMINATION OF NUCLEAR FUEL BURNUP FROM FISSION PRODUCT ANALYSES
    LISMAN, FL
    MAECK, WJ
    REIN, JE
    [J]. ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 1969, (SEP): : NU48 - &
  • [6] DETERMINATION OF NUCLEAR FUEL BURNUP FROM FISSION PRODUCT ANALYSIS
    LISMAN, FL
    MAECK, WJ
    REIN, JE
    [J]. NUCLEAR SCIENCE AND ENGINEERING, 1970, 42 (02) : 215 - &
  • [7] Distribution of metallic fission-product particles in the cladding liner of spent nuclear fuel
    Richard A. Clark
    Michele A. Conroy
    Timothy G. Lach
    Edgar C. Buck
    Kristi L. Pellegrini
    Bruce K. McNamara
    Jon M. Schwantes
    [J]. npj Materials Degradation, 4
  • [8] Residual energy release and actinide and fission product radiotoxicities during long-term storage of high burnup spent VVER fuel
    Bergel'son, B. R.
    Gerasimov, S.
    Zaritskaya, T. S.
    Tikhomirov, G. V.
    [J]. ATOMIC ENERGY, 2007, 102 (05) : 364 - 368
  • [9] The need for speed - Burnup determination of spent nuclear fuel
    Roach, Benjamin D.
    Rogers, Kayron T.
    Zirakparvar, N. Alex
    Delashmitt, Jeffrey S.
    Metzger, Shalina C.
    Manard, Benjamin T.
    Keever, Tamara J.
    Giaquinto, Joseph M.
    Hexel, Cole
    [J]. TALANTA OPEN, 2022, 6
  • [10] Determination of the Burnup of Spent Nuclear Fuel during Reloading
    S. G. Oleinik
    M. V. Maksimov
    O. V. Maslov
    [J]. Atomic Energy, 2002, 92 : 296 - 300
12345