Determination of actinide and fission-product isotopes in very-high-burnup spent nuclear fuel

被引：9

作者：

Sullivan, V. S. ^{[1
]}

Bowers, D. L. ^{[1
]}

Clark, M. A. ^{[1
]}

Graczyk, D. G. ^{[1
]}

Tsai, Y. ^{[1
]}

Streets, W. E. ^{[1
]}

Pol, M. H. Vander ^{[1
]}

Billone, M. C. ^{[2
]}

机构：

[1] Argonne Natl Lab, Div Chem Engn, Argonne, IL 60439 USA

[2] Argonne Natl Lab, Div Energy Technol, Argonne, IL 60439 USA

来源：

JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY | 2008年 / 277卷 / 01期

关键词：

Plutonium; Thermal Ionization Mass Spectrometry; Nuclear Regulatory Commission; Chemical Engineer Division; Separate Rare Earth;

D O I：

10.1007/s10967-008-0709-4

中图分类号：

O65 [分析化学];

学科分类号：

070302 ; 081704 ;

摘要：

A work plan was desired that would produce data for a wide array of actinide and fission-product isotopes with reasonably good accuracy and relatively low cost. An analysis scheme involving a fairly small number of separations, dilutions, and measurement methods was used to generate information on 74 isotopes in two spent-fuel samples of > 70 GWd/MTU burnup. Some of the measured isotopes are of high interest for burnup-credit evaluations and had not been reported previously for high-burnup fuels.

引用

页码：59 / 64

页数：6

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