Determination of actinide and fission-product isotopes in very-high-burnup spent nuclear fuel

被引:0
|
作者
V. S. Sullivan
D. L. Bowers
M. A. Clark
D. G. Graczyk
Y. Tsai
W. E. Streets
M. H. Vander Pol
M. C. Billone
机构
[1] Argonne National Laboratory,Chemical Engineering Division
[2] Argonne National Laboratory,Energy Technology Division
关键词
Plutonium; Thermal Ionization Mass Spectrometry; Nuclear Regulatory Commission; Chemical Engineer Division; Separate Rare Earth;
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学科分类号
摘要
A work plan was desired that would produce data for a wide array of actinide and fission-product isotopes with reasonably good accuracy and relatively low cost. An analysis scheme involving a fairly small number of separations, dilutions, and measurement methods was used to generate information on 74 isotopes in two spent-fuel samples of >70 GWd/MTU burnup. Some of the measured isotopes are of high interest for burnup-credit evaluations and had not been reported previously for high-burnup fuels.
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页码:59 / 64
页数:5
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