Water-Stable Anionic Metal-Organic Framework for Highly Selective Separation of Methane from Natural Gas and Pyrolysis Gas

被引：144
|
作者：
Li, Lan [1 ,2 ]
Wang, Xusheng [2 ]
Liang, Jun [2 ]
Huang, Yuanbiao [2 ]
Li, Hongfang [2 ]
Lin, Zujin [2 ]
Cao, Rong [1 ,2 ]
机构：
[1] Univ Sci & Technol China, Dept Chem, Hefei 230026, Anhui, Peoples R China
[2] Chinese Acad Sci, Fujian Inst Res Struct Matter, State Key Lab Struct Chem, Fuzhou 350002, Fujian, Peoples R China
来源：
ACS APPLIED MATERIALS & INTERFACES | 2016年 / 8卷 / 15期
关键词：
MOFs; phosphorus; light hydrocarbons; selectivity; water-stable; adsorption; CARBON-DIOXIDE CAPTURE; LIGHT-HYDROCARBONS; COORDINATION SITES; CO2; ADSORPTION; CONSTRUCTION; ACETYLENE; SORPTION; STORAGE; LIGAND; ENERGY;
D O I：
10.1021/acsami.6b00706
中图分类号：
TB3 [工程材料学];
学科分类号：
0805 ; 080502 ;
摘要：
A 3D water-stable anionic metal-organic framework [Zn-4(hpdia)(2)]center dot[NH2(CH3)(2)]center dot 3DMF center dot 4H(2)O (FJI-C4) was constructed based on an elaborate phosphorus-containing ligand 5,5'-(hydroxyphosphoryl)diisophthalic acid (H(5)hpdia). FJI-C4 with narrow one-dimensional (1D) pore channels exhibits high selectivity of C3H8/CH4 and C2H2/CH4. It is the first time for the MOF which contains phosphorus for selective separation of methane from natural gas and pyrolysis gas.
引用
收藏
页码：9777 / 9781
页数：5
相关论文
共 50 条
  • [31] A water-stable luminescent cadmium-thiazole metal-organic framework for detection of some anionic and aromatic pollutants
    Hosseini, Akram Karbalaee
    Pourshirzad, Yasaman
    Tadjarodi, Azadeh
    [J]. JOURNAL OF SOLID STATE CHEMISTRY, 2023, 317
  • [32] A Combinatorial Approach towards Water-Stable Metal-Organic Frameworks for Highly Efficient Carbon Dioxide Separation
    Hu, Zhigang
    Zhang, Kang
    Zhang, Mei
    Guo, Zhengang
    Jiang, Jianwen
    Zhao, Dan
    [J]. CHEMSUSCHEM, 2014, 7 (10) : 2791 - 2795
  • [33] Highly Water-Stable Zinc Based Metal-Organic Framework: Antibacterial, Photocatalytic Degradation and Photoelectric Responses
    Yuan, Congying
    Miao, Yadi
    Chai, Yinhang
    Zhang, Xiaojun
    Dong, Xiaojing
    Zhao, Ying
    [J]. MOLECULES, 2023, 28 (18):
  • [34] A Microporous Metal-Organic Framework for Highly Selective Separation of Acetylene, Ethylene, and Ethane from Methane at Room Temperature
    He, Yabing
    Zhang, Zhangjing
    Xiang, Shengchang
    Fronczek, Frank R.
    Krishna, Rajamani
    Chen, Banglin
    [J]. CHEMISTRY-A EUROPEAN JOURNAL, 2012, 18 (02) : 613 - 619
  • [35] Highly selective capture of phosphate ions from water by a water stable metal-organic framework modified with polyethyleneimine
    Qiu, Hui
    Yang, Luyang
    Liu, Fengling
    Zhao, Yunxia
    Liu, LeLe
    Zhu, Jinhong
    Song, Mingxia
    [J]. ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH, 2017, 24 (30) : 23694 - 23703
  • [36] Highly selective capture of phosphate ions from water by a water stable metal-organic framework modified with polyethyleneimine
    Hui Qiu
    Luyang Yang
    Fengling Liu
    Yunxia Zhao
    LeLe Liu
    Jinhong Zhu
    Mingxia Song
    [J]. Environmental Science and Pollution Research, 2017, 24 : 23694 - 23703
  • [37] Highly porous metal-organic framework glass design and application for gas separation membranes
    Shichun Li
    Chao Ma
    Jingwei Hou
    Shuwen Yu
    Aibing Chen
    Juan Du
    Philip A. Chater
    Dean S. Keeble
    Zhihua Qiao
    Chongli Zhong
    David A. Keen
    Yu Liu
    Thomas D. Bennett
    [J]. Nature Communications, 16 (1)
  • [38] Highly selective gas separation membrane using in situ amorphised metal-organic frameworks
    Kertik, Aylin
    Wee, Lik H.
    Pfannmoeller, Martin
    Bals, Sara
    Martens, Johan A.
    Vankelecom, Ivo F. J.
    [J]. ENERGY & ENVIRONMENTAL SCIENCE, 2017, 10 (11) : 2342 - 2351
  • [39] A Highly Water-Stable meta-Carborane-Based Copper Metal-Organic Framework for Efficient High-Temperature Butanol Separation
    Gan, Lei
    Chidambaram, Arunraj
    Fonquernie, Pol G.
    Light, Mark E.
    Choquesillo-Lazarte, Duane
    Huang, Hongliang
    Solano, Eduardo
    Fraile, Julio
    Vinas, Clara
    Teixidor, Francesc
    Navarro, Jorge A. R.
    Stylianou, Kyriakos C.
    Planas, Jose G.
    [J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2020, 142 (18) : 8299 - 8311
  • [40] High proton conduction in an excellent water-stable gadolinium metal-organic framework
    Xing, Xiu-Shuang
    Fu, Zhi-Hua
    Zhang, Ning-Ning
    Yu, Xiao-Qing
    Wang, Ming-Sheng
    Guo, Guo-Cong
    [J]. CHEMICAL COMMUNICATIONS, 2019, 55 (09) : 1241 - 1244
12345