A significant difference between the transient electric field profiles of the pentacene organic field-effect transistors (OFETs) with SiO(2) and poly(methyl-methacrylate) (PMMA) insulators was found by the time-resolved microscopic optical second-harmonic generation (TRM-SHG) experiment. The profile of former device was broad and changed smoothly, while the latter one had a sharp peak. Particularly, the peak of the transient electric field in SiO(2)-insulated devices moved much faster than that in the PMMA-insulated one. Based on several experimental evidences and computational simulations, we proposed that these differences might arise from a higher trapped carrier density in the conductive channel on the PMMA insulator. Simple approaches were developed to evaluate the trap density and define dynamic carrier mobility in terms of the transient electric field measured by the TRM-SHG technique. This mobility quantitatively depicts that the transient hole transport in the OFET with the PMMA insulator is trap controlled.
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NIST, Div Engn Phys, 100 Bur Dr,MS 8120, Gaithersburg, MD 20899 USA
Wake Forest Univ, Dept Phys, 1834 Wake Forest Rd, Winston Salem, NC 27109 USANIST, Div Engn Phys, 100 Bur Dr,MS 8120, Gaithersburg, MD 20899 USA
Bittle, Emily G.
Basham, James I.
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NIST, Div Engn Phys, 100 Bur Dr,MS 8120, Gaithersburg, MD 20899 USA
Penn State Univ, Dept Elect Engn, 121 Elect Engn East, State Coll, PA 16802 USANIST, Div Engn Phys, 100 Bur Dr,MS 8120, Gaithersburg, MD 20899 USA
Basham, James I.
Jackson, Thomas N.
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Penn State Univ, Dept Elect Engn, 121 Elect Engn East, State Coll, PA 16802 USANIST, Div Engn Phys, 100 Bur Dr,MS 8120, Gaithersburg, MD 20899 USA
Jackson, Thomas N.
Jurchescu, Oana D.
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Wake Forest Univ, Dept Phys, 1834 Wake Forest Rd, Winston Salem, NC 27109 USANIST, Div Engn Phys, 100 Bur Dr,MS 8120, Gaithersburg, MD 20899 USA
Jurchescu, Oana D.
Gundlach, David J.
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NIST, Div Engn Phys, 100 Bur Dr,MS 8120, Gaithersburg, MD 20899 USANIST, Div Engn Phys, 100 Bur Dr,MS 8120, Gaithersburg, MD 20899 USA
机构:
Key Laboratory of Micro and Nano Photonic Structures (Ministry of Education) and State Key Laboratory of Surface Physics,Fudan UniversityKey Laboratory of Micro and Nano Photonic Structures (Ministry of Education) and State Key Laboratory of Surface Physics,Fudan University
何鋆
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陈小青
侯晓远
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Key Laboratory of Micro and Nano Photonic Structures (Ministry of Education) and State Key Laboratory of Surface Physics,Fudan UniversityKey Laboratory of Micro and Nano Photonic Structures (Ministry of Education) and State Key Laboratory of Surface Physics,Fudan University