Fully Transparent Quantum Dot Light-Emitting Diode with a Laminated Top Graphene Anode

被引:40
|
作者
Yao, Li [1 ]
Fang, Xin [1 ]
Gu, Wei [2 ,3 ]
Zhai, Wenhao [1 ]
Wan, Yi [1 ]
Xie, Xixi [1 ]
Xu, Wanjin [1 ]
Pi, Xiaodong [2 ,3 ]
Ran, Guangzhao [1 ]
Qin, Guogang [1 ]
机构
[1] Peking Univ, Sch Phys, State Key Lab Microscop Phys, Beijing 100871, Peoples R China
[2] Zhejiang Univ, State Key Lab Silicon Mat, Hangzhou 310027, Zhejiang, Peoples R China
[3] Zhejiang Univ, Sch Mat Sci & Engn, Hangzhou 310027, Zhejiang, Peoples R China
基金
中国国家自然科学基金;
关键词
graphene; transparent top electrode; lamination; quantum dots; light emitting diodes; SINGLE-LAYER GRAPHENE; EFFICIENT; DEVICE; BRIGHT; ELECTRODES; FILMS;
D O I
10.1021/acsami.7b02026
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
A new method to employ graphene as top electrode was introduced, and based on that, fully transparent quantum dot light-emitting diodes (T-QLEDs) were successfully fabricated through a lamination process. We adopted the widely used wet transfer method to transfer bilayer graphene (BG) on polydimethylsiloxane/polyethylene terephthalate (PDMS/PET) substrate. The sheet resistance of graphene reduced to,,540 WO through transferring BG for 3 times on the PDMS/PET. The T-QLED has an inverted device structure of glass/indium tin oxide (ITO)/ZnO nanoparticles/(CdSSe/ZnS quantum dots (QDs))/1,1-bis[(di-4tolylamitio)phenyl] cyclohexane (TAPC)/MoO3/graphene/ PDMS/PET. The graphene anode on PDMS/PET substrate can be directly laminated on the MoO3/TAPC/(CdSSe/ZnS QDs)/ZnO nanoparticles/ITO/glass, which relied on the van der Waals interaction between the graphene/PDMS and the MoO3. The transmittance of the T-QLED is 79.4% at its main electroluminescence peak wavelength of 622 run.
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页码:24005 / 24010
页数:6
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