Rational Syntheses of CdII and PbII Metal-Organic Frameworks for Luminescence Sensing of Nitroaromatics, Ferric and Chromate Ions

被引：15

作者：

Wu, Yu ^{[1
]}

Li, Yulong ^{[1
]}

Zou, Like ^{[1
]}

Feng, Jianshen ^{[1
]}

Liu, Jianqiang ^{[2
]}

Luo, Miaomiao ^{[2
]}

Xu, Jingwen ^{[2
]}

Yadav, Reena ^{[3
]}

Kumar, Abhinav ^{[3
]}

机构：

[1] Sichuan Univ Sci & Engn, Coll Chem & Environm Engn, Zigong 643000, Peoples R China

[2] Guangdong Med Univ, Sch Pharm, Dongguan 523808, Peoples R China

[3] Univ Lucknow, Fac Sci, Dept Chem, Lucknow 226007, Uttar Pradesh, India

来源：

ZEITSCHRIFT FUR ANORGANISCHE UND ALLGEMEINE CHEMIE | 2017年 / 643卷 / 02期

基金：

中国国家自然科学基金;

关键词：

Coordination polymer; Photoluminescence; Sensing; Topology; Density functional calculations; COMPLEXES; LIGANDS; SENSOR; MOF; EXPLOSIVES; FE(III); ACETONE; BLOCKS;

D O I：

10.1002/zaac.201600344

中图分类号：

O61 [无机化学];

学科分类号：

070301 ; 081704 ;

摘要：

The metal-organic frameworks (MOFs), {[Cd(L)(H2O)]CH3OHDMF} (1) and [Pb(L)(DMF)] (2) (L = 2,4-dihydroxybenzaldehyde nicotinoylhydrazone), were synthesized and characterized using microanalyses, IR spectroscopy, and single-crystal X-ray diffraction. Single crystal X-ray analyses revealed that both 1 and 2 exhibit 2D grid networks. The photoluminescence investigation indicates that 1 and 2 could be a prospective candidate for developing luminescencent sensors for the selective sensing of nitrobenzene, which is used as a precursor for explosives. The luminescent properties of 1 and 2 in different solvents were investigated and corroborated by theoretical calculations. Additionally compounds 1 and 2 also show selective sensing ability for Fe3+ as well as for CrO42- ions.

引用

页码：214 / 219

页数：6

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