Production of high purity hydrogen by ethanol steam reforming in membrane reactor

被引：47

作者：

Mironova, E. Yu. ^{[1
]}

Ermilova, M. M. ^{[1
]}

Orekhova, N. V. ^{[1
]}

Muraviev, D. N. ^{[2
]}

Yaroslavtsev, A. B. ^{[1
,3
]}

机构：

[1] Russian Acad Sci, AV Topchiev Inst Petrochem Synth, Moscow 119991, Russia

[2] UAB, Dept Chem, Anal Chem Unit, Bellaterra 08193, Barcelona, Spain

[3] Moscow MV Lomonosov State Univ, Dept Chem, Moscow 119991, Russia

来源：

CATALYSIS TODAY | 2014年 / 236卷

关键词：

Ethanol steam reforming; Pd-Ru membrane reactor; Nanodiamond-supported metal catalysts; POLYMER ELECTROLYTE MEMBRANES; BIO-ETHANOL; NANOCATALYSTS; TEMPERATURE; CONVERSION; BIOMASS;

D O I：

10.1016/j.cattod.2014.01.014

中图分类号：

O69 [应用化学];

学科分类号：

081704 ;

摘要：

Production of hydrogen in the course of ethanol steam reforming (ESR) on bimetallic Pt-Ni and Pt-Ru nanocatalysts supported on detonation nanodiamonds (DND) was studied in conventional and membrane reactors. The highest hydrogen yield and purity were achieved in the case of Pt-Ru/DND catalysts at total metal content of 0.3% and atomic Pt/Ru ratio of 911. It is shown that realization of ESR process in the membrane reactor with simultaneous hydrogen removal through the Pd-Ru membrane produces hydrogen of high purity, free of any other gaseous products. (C) 2014 Elsevier B.V. All rights reserved.

引用

页码：64 / 69

页数：6

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