Redistributed Current Density in Lateral Organic Light-Emitting Transistors Enabling Uniform Area Emission with Good Stability and Arbitrary Tunability

被引:57
|
作者
Gao, Haikuo [1 ,2 ,3 ]
Miao, Zhagen [1 ,3 ]
Qin, Zhengsheng [1 ,3 ]
Yang, Jiaxin [1 ,3 ]
Wang, Tianyu [1 ]
Gao, Can [1 ]
Dong, Huanli [1 ]
Hu, Wenping [4 ]
机构
[1] Chinese Acad Sci, Inst Chem, Key Lab Organ Solids, Beijing Natl Lab Mol Sci, Beijing 100190, Peoples R China
[2] Binzhou Univ, Coll Aeronaut Engn, Shandong Engn Res Ctr Aeronaut Mat & Devices, Binzhou 251900, Peoples R China
[3] Univ Chinese Acad Sci, Sch Chem Sci, Beijing 100049, Peoples R China
[4] Tianjin Univ, Sch Sci, Collaborat Innovat Ctr Chem Sci & Engn, Dept Chem, Tianjin 300072, Peoples R China
基金
中国国家自然科学基金;
关键词
area emission; charge-transport buffer layers; lateral geometry; organic light-emitting transistors; redistributed current density; FIELD-EFFECT TRANSISTORS; LOW-VOLTAGE; AMBIPOLAR; EFFICIENCY; DEVICE; GATE;
D O I
10.1002/adma.202108795
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Organic light-emitting transistors (OLETs), integrating the functions of an organic field-effect transistor (OFET) and organic light-emitting diode (OLED) in a single device, are promising for the next-generation display technology. However, the great challenge of achieving uniform area emission in OLETs with good stability and arbitrary tunability hinders their development in this field. Herein, an effective solution to obtain well-defined area emission in lateral OLETs by incorporating a charge-transport buffer (CTB) layer between the conducting channel and emitting layer is proposed. Comprehensive theoretical simulation and experimental results demonstrate redistributed potential beneath the drain electrode under the shielding effect of the CBT layer, resulting in a highly uniform current density. In this case, uniform recombination of balanced holes and electrons can be guaranteed, which is essential for the formation of area emission in the following OLETs. RGB OLETs with uniform area emission are constructed, which show good gate tunable ability (ON/OFF ratio 10(6)), high loop stability (over 200 cycles) and high aperture ratio (over 80%) due to the arbitrary tunability of the device geometry. This work provides a new avenue for constructing area-emission lateral OLETs, which have great potential for display technology because of their good compatibility with conventional fabrication techniques.
引用
收藏
页数:9
相关论文
共 50 条
  • [1] High current density in light-emitting transistors of organic single crystals
    Takenobu, Taishi
    Bisri, Satria Zulkarnaen
    Takahashi, Tetsuo
    Yahiro, Masayuki
    Adachi, Chihaya
    Iwasa, Yoshihiro
    PHYSICAL REVIEW LETTERS, 2008, 100 (06)
  • [2] Current-Confinement Structure and Extremely High Current Density in Organic Light-Emitting Transistors
    Sawabe, Kosuke
    Imakawa, Masaki
    Nakano, Masaki
    Yamao, Takeshi
    Hotta, Shu
    Iwasa, Yoshihiro
    Takenobu, Taishi
    ADVANCED MATERIALS, 2012, 24 (46) : 6141 - 6146
  • [3] High Efficiency and Uniform Emission in Micropixelated Inorganic/ Organic Hybrid Vertical Light-Emitting Transistors and Displays
    Chang, Jui-Fen
    Huang, Guang-Ru
    Wu, Yu-Pei
    Chang, Chih-Hao
    Lo, Yu-Jen
    Yu, Jia-Min
    ACS APPLIED ELECTRONIC MATERIALS, 2022, 4 (12) : 5752 - 5762
  • [4] Separation in the Roles of Carrier Transport and Light Emission in Light-Emitting Organic Transistors with a Bilayer Configuration
    Shang, Hui
    Shimotani, Hidekazu
    Kanagasekaran, Thangavel
    Tanigaki, Katsumi
    ACS APPLIED MATERIALS & INTERFACES, 2019, 11 (22) : 20200 - 20204
  • [5] Quasi-surface emission in vertical organic light-emitting transistors with network electrode
    Keum, Chang-Min
    Lee, In-Ho
    Lee, Sin-Hyung
    Lee, Gyu Jeong
    Kim, Min-Hoi
    Lee, Sin-Doo
    OPTICS EXPRESS, 2014, 22 (12): : 14750 - 14756
  • [6] Ag fiber/IZO Composite Electrodes: Improved Chemical and Thermal Stability and Uniform Light Emission in Flexible Organic Light-Emitting Diodes
    Choi, Junhee
    Park, Cheol Hwee
    Kwack, Jin Ho
    Lee, Dong Jun
    Kim, Jae Geun
    Choi, Jaemyeong
    Bae, Bong Han
    Park, Soo Jong
    Kim, Enjung
    Park, Young Wook
    Ju, Byeong-Kwon
    SCIENTIFIC REPORTS, 2019, 9 (1)
  • [7] Ag fiber/IZO Composite Electrodes: Improved Chemical and Thermal Stability and Uniform Light Emission in Flexible Organic Light-Emitting Diodes
    Junhee Choi
    Cheol Hwee Park
    Jin Ho Kwack
    Dong Jun Lee
    Jae Geun Kim
    Jaemyeong Choi
    Bong Han Bae
    Soo Jong Park
    Enjung Kim
    Young Wook Park
    Byeong-Kwon Ju
    Scientific Reports, 9
  • [8] Effects of disorder on the current density and recombination profile in organic light-emitting diodes
    Coehoorn, R.
    van Mensfoort, S. L. M.
    PHYSICAL REVIEW B, 2009, 80 (08)
  • [9] High Mobility Organic Lasing Semiconductor with Crystallization-Enhanced Emission for Light-Emitting Transistors
    Liu, Dan
    Liao, Qing
    Peng, Qian
    Gao, Haikuo
    Sun, Qi
    De, Jianbo
    Gao, Can
    Miao, Zhagen
    Qin, Zhengsheng
    Yang, Jiaxin
    Fu, Hongbing
    Shuai, Zhigang
    Dong, Huanli
    Hu, Wenping
    ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2021, 60 (37) : 20274 - 20279
  • [10] Organic light-emitting transistors with voltage-tunable lit area and full channel illumination
    Toffanin, Stefano
    Capelli, Raffaella
    Koopman, Wouter
    Generali, Gianluca
    Cavallini, Susanna
    Stefani, Andrea
    Saguatti, Davide
    Ruani, Giampiero
    Muccini, Michele
    LASER & PHOTONICS REVIEWS, 2013, 7 (06) : 1011 - 1019