Exciton fine structure splitting and linearly polarized emission in strained transition-metal dichalcogenide monolayers

被引:9
|
作者
Glazov, M. M. [1 ,2 ]
Dirnberger, Florian [3 ,4 ,5 ,6 ]
Menon, Vinod M. [3 ,4 ]
Taniguchi, Takashi [7 ]
Watanabe, Kenji [8 ]
Bougeard, Dominique [9 ]
Ziegler, Jonas D. [5 ,6 ,10 ]
Chernikov, Alexey [5 ,6 ,10 ]
机构
[1] Ioffe Inst, St Petersburg 194021, Russia
[2] Natl Res Univ, Higher Sch Econ, St Petersburg 190121, Russia
[3] CUNY City Coll, Dept Phys, New York, NY 10031 USA
[4] City Univ New York, Grad Ctr, Dept Phys, New York, NY 10016 USA
[5] Tech Univ Dresden, Inst Appl Phys, Integrated Ctr Appl Phys & Photon Mat, D-01062 Dresden, Germany
[6] Tech Univ Dresden, Wurzburg Dresden Cluster Excellence Ct Qmat, D-01062 Dresden, Germany
[7] Natl Inst Mat Sci, Int Ctr Mat Nanoarchitecton, Tsukuba, Ibaraki 305004, Japan
[8] Natl Inst Mat Sci, Res Ctr Funct Mat, Tsukuba, Ibaraki 305004, Japan
[9] Univ Regensburg, Dept Phys, D-93040 Regensburg, Germany
[10] Tech Univ Dresden, Wurzburg Dresden Cluster Excellence ct qmat, Internationa Ctr Appl Phys & Photon Mat, Wurzburg-Dresden Cluster Excellence ct, D-01062 Dresden, Germany
关键词
EXCHANGE INTERACTION; VALLEY POLARIZATION; SPIN; MOS2; DYNAMICS; HEAVY;
D O I
10.1103/PhysRevB.106.125303
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We study theoretically the effects of an anisotropic elastic strain on the exciton energy spectrum fine structure and optical selection rules in atomically thin crystals based on transition-metal dichalcogenides. The presence of strain breaks the chiral selection rules at the K points of the Brillouin zone and makes optical transitions linearly polarized. The orientation of the induced linear polarization is related to the main axes of the strain tensor. Elastic strain provides an additive contribution to the exciton fine structure splitting, in agreement with experimental evidence obtained from the uniaxially strained WSe2 monolayer. The applied strain also induces momentum-dependent Zeeman splitting. Depending on the strain orientation and magnitude, Dirac points with a linear dispersion can be formed in the exciton energy spectrum. We provide a symmetry analysis of the strain effects and develop a microscopic theory for all relevant strain-induced contributions to the exciton fine structure Hamiltonian.
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页数:11
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