"Click Chemistry" Mediated Functional Microporous Organic Nanotube Networks for Heterogeneous Catalysis

被引：21

作者：

Yu, Wei ^{[1
]}

Zhou, Minghong ^{[1
]}

Wang, Tianqi ^{[1
]}

He, Zidong ^{[1
]}

Shi, Buyin ^{[1
]}

Xu, Yang ^{[1
]}

Huang, Kun ^{[1
]}

机构：

[1] East China Normal Univ, Sch Chem & Mol Engn, 500 N,Dongchuan Rd, Shanghai 200241, Peoples R China

来源：

ORGANIC LETTERS | 2017年 / 19卷 / 21期

基金：

美国国家科学基金会;

关键词：

HIGH-SURFACE-AREA; HYPERCROSSLINKED POLYMERS; NUCLEOPHILIC CATALYST; HOMOGENEOUS CATALYSTS; RECYCLABLE CATALYSTS; MESOPOROUS SILICA; AEROBIC OXIDATION; POROUS POLYMERS; SUPPORTED TEMPO; CO2; CAPTURE;

D O I：

10.1021/acs.orglett.7b02682

中图分类号：

O62 [有机化学];

学科分类号：

070303 ; 081704 ;

摘要：

The synthesis of azide functional microporous organic nanotube networks (N-3-MONNs) via a Friedel Crafts hyper-cross linking reaction is reported. Subsequently, a general method for obtaining heterogeneous catalysts through a Cu-catalyzed alkyne azide reaction is presented. The small-molecule catalysts such as 2,2,6,6,tetramethylpiperidine-1-oyl and 4-(N,N-dimethylamino)pyridine can be anchored into the MONNs. Owing to the hierarchically porous structure and high surface area, these catalysts show high activity in selective oxidation of alcohols and acylation reaction, respectively.

引用

页码：5776 / 5779

页数：4

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