Optical absorption measurements of electron quantum confinement in Si(111)-2x1 surface chains

被引:3
|
作者
Bussetti, G. [1 ,2 ]
Violante, A. [1 ,2 ]
Bonanni, B. [1 ,2 ]
Cirilli, S. [1 ,2 ]
Goletti, C. [1 ,2 ]
Chiaradia, P. [1 ,2 ]
Chiarotti, G. [1 ,2 ]
Rohlfing, M. [3 ]
机构
[1] Univ Roma Tor Vergata, Dipartimento Fis, NAST, I-00173 Rome, Italy
[2] Univ Roma Tor Vergata, CNISM, I-00173 Rome, Italy
[3] Univ Osnabruck, Fachbereich Phys, D-4500 Osnabruck, Germany
关键词
EXCITONS; OXYGEN;
D O I
10.1103/PhysRevB.82.153304
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Optical experiments on the Si(111)-2x1 surface show that the absorption peak due to dangling-bond transitions exhibits a blueshift upon oxygen exposure. The effect is interpreted as due to quantum confinement of surface electrons in pi-bonded chains of atoms, whose length decreases with oxygen uptake (a particle-in-a-box effect, the box being one dimensional). This conclusion is supported by numerical simulation of the optical spectra.
引用
收藏
页数:4
相关论文
共 50 条
  • [21] Microscopic theory for the nonlinear optical response of the Si(111)-(2x1) surface exciton
    Reichelt, M
    Meier, T
    Rohlfing, M
    Koch, SW
    PHYSICA STATUS SOLIDI B-BASIC RESEARCH, 2003, 238 (03): : 525 - 528
  • [22] THE MOTT INSULATOR MODEL OF THE SI(111)-(2X1) SURFACE
    REDONDO, A
    GODDARD, WA
    MCGILL, TC
    SURFACE SCIENCE, 1983, 132 (1-3) : 49 - 61
  • [23] Electrostatics and reactivity of surface defects on Si(111)-(2X1)
    Kádas, K
    Náray-Szabó, G
    JOURNAL OF MOLECULAR STRUCTURE-THEOCHEM, 1998, 455 (2-3): : 213 - 218
  • [24] TEST OF STRUCTURAL MODELS FOR THE SI(111)2X1 SURFACE
    LIU, H
    COOK, MR
    JONA, F
    MARCUS, PM
    PHYSICAL REVIEW B, 1983, 28 (10): : 6137 - 6140
  • [25] SURFACE BAND-STRUCTURE OF SI(111)2X1
    CHEN, B
    HANEMAN, D
    PHYSICAL REVIEW B, 1995, 51 (07): : 4258 - 4263
  • [26] MOTT INSULATOR MODEL OF THE SI(111)-(2X1) SURFACE
    REDONDO, A
    GODDARD, WA
    MCGILL, TC
    JOURNAL OF VACUUM SCIENCE & TECHNOLOGY, 1982, 21 (02): : 328 - 329
  • [27] Band structure of the Ca/Si(111)-(2x1) surface
    Sakamoto, K
    Zhang, HM
    Uhrberg, RIG
    PHYSICAL REVIEW B, 2003, 68 (24):
  • [28] DIPOLE ACTIVITY OF SURFACE PHONONS ON SI(111)2X1
    ALERHAND, OL
    ALLAN, DC
    MELE, EJ
    PHYSICAL REVIEW LETTERS, 1985, 55 (24) : 2700 - 2703
  • [29] Dimerized, buckled, or ideal chains on the diamond (111)2x1 surface?
    Schmidt, WG
    Scholze, A
    Bechstedt, F
    SURFACE SCIENCE, 1996, 351 (1-3) : 183 - 188
  • [30] SURFACE-STATE OPTICAL-ABSORPTION ON THE CLEAN SI(100)2X1 SURFACE
    CHABAL, YJ
    CHRISTMAN, SB
    CHABAN, EE
    YIN, MT
    JOURNAL OF VACUUM SCIENCE & TECHNOLOGY A-VACUUM SURFACES AND FILMS, 1983, 1 (02): : 1241 - 1242