Recent Progress on Establishing Structure-Activity Relationship of Catalysts for Selective Catalytic Reduction (SCR) of NOx with NH3

被引:20
|
作者
Huang, Xiaosheng [1 ,2 ]
Zhang, Guodong [1 ]
Lu, Gongxuan [1 ]
Tang, Zhicheng [1 ]
机构
[1] Chinese Acad Sci, Lanzhou Inst Chem Phys, State Key Lab Oxo Synth & Select Oxidat, Natl Engn Res Ctr Fine Petrochem Intermediates, Lanzhou 730000, Gansu, Peoples R China
[2] Univ Chinese Acad Sci, Beijing 100039, Peoples R China
基金
中国科学院西部之光基金; 中国国家自然科学基金;
关键词
SCR catalyst; NOx control; Structure-activity relationship; Reaction mechanism; Research progress; MIXED-OXIDE CATALYST; LOW-TEMPERATURE SCR; NITRIC-OXIDE; NH3-SCR REACTION; NITROGEN-OXIDES; CHEMICAL DEACTIVATION; COMMERCIAL CATALYSTS; MNOX-CEO2; MECHANISM; MESOPOROUS SILICA; LUBRICATION OILS;
D O I
10.1007/s10563-017-9237-y
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Catalytic elimination is an important technique to reduce the emission of atmospheric molecular contaminants (such as NOx) efficiently. Selective catalytic reduction (SCR) is one of the most important nitrogen oxide (NOx) control technologies in the world, and catalyst plays a greatly important role in SCR process. In this field, the novel catalysts and preparation methods have attracted more and more attention in recent years due to their excellent catalytic performance. It is well accepted that catalytic performance is significantly dependent on the supports, active sites, and interaction of support and active component of the catalysts. In this paper, we present a brief review on the preparation methods of different kinds of SCR catalysts in recent years and propose some perspectives for further development. Based on the report of published literatures, the structure-activity relationship between support and active sites is deeply analyzed. Meanwhile, we review the possible catalytic mechanism, and further clarify the nature of the catalytic reactions.
引用
收藏
页码:1 / 19
页数:19
相关论文
共 50 条
  • [1] Recent Progress on Establishing Structure–Activity Relationship of Catalysts for Selective Catalytic Reduction (SCR) of NOx with NH3
    Xiaosheng Huang
    Guodong Zhang
    Gongxuan Lu
    Zhicheng Tang
    Catalysis Surveys from Asia, 2018, 22 : 1 - 19
  • [2] Structure-Activity Relationship of Iron Titanate Catalysts in the Selective Catalytic Reduction of NOx with NH3
    Liu, Fudong
    He, Hong
    JOURNAL OF PHYSICAL CHEMISTRY C, 2010, 114 (40): : 16929 - 16936
  • [3] Recent progress in the selective catalytic reduction of NOx with NH3 on Cu-SAPO-34 catalysts
    Jablonska, Magdalena
    MOLECULAR CATALYSIS, 2022, 518
  • [4] Selective Catalytic Reduction (SCR) of NOx with NH3 on Sb-promoted VWTi Catalysts
    Kim, Su Bin
    Choi, Gyeong Ryun
    Shin, Jung Hun
    Hong, Sung Chang
    APPLIED CHEMISTRY FOR ENGINEERING, 2021, 32 (01): : 35 - 41
  • [5] Research Progress of Ceria-Based Catalysts in the Selective Catalytic Reduction of NOx by NH3
    Yao Xiao-Jiang
    Gong Ying-Tao
    Li Hong-Li
    Yang Fu-Mo
    ACTA PHYSICO-CHIMICA SINICA, 2015, 31 (05) : 817 - 828
  • [6] Recent Progress of CeO2-TiO2 Based Catalysts for Selective Catalytic Reduction of NOx by NH3
    Zeng, Yiqing
    Haw, Kok-Giap
    Wang, Yanan
    Zhang, Shule
    Wang, Zhigang
    Zhong, Qin
    Kawi, Sibudjing
    CHEMCATCHEM, 2021, 13 (02) : 491 - 505
  • [7] Research Progress in Iron-Based Catalysts for the Selective Catalytic Reduction of NOx by NH3
    Zhang Hong-Liang
    Long Hong-Ming
    Li Jia-Xin
    Dong Lin
    CHINESE JOURNAL OF INORGANIC CHEMISTRY, 2019, 35 (05) : 753 - 768
  • [8] Recent advances in the selective catalytic reduction of NOx with NH3 on Cu-Chabazite catalysts
    Wang, Jihui
    Zhao, Huawang
    Haller, Gary
    Li, Yongdan
    APPLIED CATALYSIS B-ENVIRONMENTAL, 2017, 202 : 346 - 354
  • [9] Catalysts for the selective catalytic reduction of NOx with NH3 at low temperature
    Shan, Wenpo
    Song, Hua
    CATALYSIS SCIENCE & TECHNOLOGY, 2015, 5 (09) : 4280 - 4288
  • [10] Fe-Ti spinel for the selective catalytic reduction of NO with NH3: Mechanism and structure-activity relationship
    Yang, Shijian
    Li, Junhua
    Wang, Chizhong
    Chen, Jinghuan
    Ma, Lei
    Chang, Huazhen
    Chen, Liang
    Peng, Yue
    Yan, Naiqiang
    APPLIED CATALYSIS B-ENVIRONMENTAL, 2012, 117 : 73 - 80