Surface-initiated reversible addition-fragmentation chain transfer polymerization from "clickable" polypropylene surface modified by iodine plasma activation

被引：7

作者：

Couturaud, B.

Mas, A.

Robin, Jean J. ^{[1
]}

机构：

[1] CNRS, UMR 5253, Inst Charles Gerhardt, F-34095 Montpellier 5, France

来源：

EUROPEAN POLYMER JOURNAL | 2015年 / 70卷

关键词：

Surface; Iodine plasma; Activation; RAFT; Grafting; RADICAL POLYMERIZATION; SUBSTRATE; POLYETHYLENE; BRUSHES; DENSITY; HYBRIDS;

D O I：

10.1016/j.eurpolymj.2015.07.019

中图分类号：

O63 [高分子化学（高聚物）];

学科分类号：

070305 ; 080501 ; 081704 ;

摘要：

An iodine modified polypropylene surface was synthesized by iodine plasma activation. The obtained polypropylene surface was found to be a useful platform for secondary reactions. For instance, an azide-functionalized PP was prepared by nucleophilic exchange reaction. The surface was proven to be reactive toward R group of an alkyne modified RAFT agent via the copper-catalyzed azide-alkyne cycloaddition. RAFT mediated graft polymerization of methacrylic acid was carried out and lead to a controlled polymerization from the surface. Characterizations of the modified surface and the grafted polymers were performed through FTIR-GATR, XPS, AFM and colorimetric assays. (C) 2015 Elsevier Ltd. All rights reserved.

引用

页码：276 / 285

页数：10

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