Controlling defects in crystalline carbon nitride to optimize photocatalytic CO2 reduction

被引：94

作者：

Li, Han ^{[1
]}

Zhu, Bicheng ^{[1
]}

Cao, Shaowen ^{[1
]}

Yu, Jiaguo ^{[1
]}

机构：

[1] Wuhan Univ Technol, State Key Lab Adv Technol Mat Synth & Proc, Wuhan 430070, Peoples R China

来源：

CHEMICAL COMMUNICATIONS | 2020年 / 56卷 / 42期

基金：

中国国家自然科学基金;

关键词：

SOLAR HYDROGEN-PRODUCTION; EXCITON DISSOCIATION; NANOSHEETS; EVOLUTION; G-C3N4;

D O I：

10.1039/d0cc01338b

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

The effective controlling of the defects of crystalline carbon nitride is presented. The rational strategy not only improves the crystallinity of carbon nitride, promoting the charge carrier transfer, but also introduces the nitrogen vacancies and cyano groups, serving as the optimal activation sites for enhanced CO2 reduction.

引用

页码：5641 / 5644

页数：4

共 50 条

[41] A Superficial Intramolecular Alignment of Carbon Nitride through Conjugated Monomer for Optimized Photocatalytic CO2 Reduction
Hayat, Asif
Sohail, Muhammad
Taha, T. A.
Alenad, Asma M.
Uddin, Ikram
Hayat, Ashiq
Ali, Tariq
Shah, Rahim
Irfan, Ahmad
Khan, Wasim Ullah
Palamanit, Arkom
Al-Hadeethi, Yas
Syed, Jawad Ali Shah
Amin, Mohammed A.
Khan, Javid
Mane, Sunil Kumar Baburao
CATALYSTS, 2021, 11 (08)
[42] Controllable adsorption groups on amine-functionalized carbon nitride for enhanced photocatalytic CO2 reduction
Cao, Shihai
Liu, Hao
Jia, Zhenhe
Guo, Meng
Gao, Wentong
Ding, Zhaohan
Yang, Weijie
Chen, Liang
Wang, Wenjing
CHEMICAL ENGINEERING JOURNAL, 2023, 455
[43] Photocatalytic reduction of CO2 by graphitic carbon nitride polymers derived from urea and barbituric acid
Qin, Jiani
Wang, Sibo
Ren, He
Hou, Yidong
Wang, Xinchen
APPLIED CATALYSIS B-ENVIRONMENTAL, 2015, 179 : 1 - 8
[44] Molecular Terpyridine-Lanthanide Complexes Modified Carbon Nitride for Enhanced Photocatalytic CO2 Reduction
Hong, Xinyue
Fang, Youting
Chao, Duobin
INORGANIC CHEMISTRY, 2024, : 12901 - 12909
[45] Construction of Carbon Nitride Based Intramolecular D-A System for Effective Photocatalytic Reduction of CO2
Zhang, Xinyu
Song, Xianghai
Yan, Yongsheng
Huo, Pengwei
CATALYSIS LETTERS, 2022, 152 (02) : 559 - 569
[46] Ultra-thin nanosheet assemblies of graphitic carbon nitride for enhanced photocatalytic CO2 reduction
Xia, Pengfei
Zhu, Bicheng
Yu, Jiaguo
Cao, Shaowen
Jaroniec, Mietek
JOURNAL OF MATERIALS CHEMISTRY A, 2017, 5 (07) : 3230 - 3238
[47] Highly crystalline carbon nitride by covalent remedy for CO2 photoreduction
Lu, Zhao
Xu, Xiutao
Wang, Zhongliao
SEPARATION AND PURIFICATION TECHNOLOGY, 2024, 330
[48] Photochemical Reduction of CO2 by Graphitic Carbon Nitride Polymers
Lin, Jinliang
Pan, Zhiming
Wang, Xinchen
ACS SUSTAINABLE CHEMISTRY & ENGINEERING, 2014, 2 (03): : 353 - 358
[49] Carbon-vacancy modified graphitic carbon nitride: enhanced CO2 photocatalytic reduction performance and mechanism probing
Shen, Meng
Zhang, Lingxia
Wang, Min
Tian, Jianjian
Jin, Xixiong
Guo, Limin
Wang, Lianzhou
Shi, Jianlin
JOURNAL OF MATERIALS CHEMISTRY A, 2019, 7 (04) : 1556 - 1563
[50] Photocatalytic CO2 reduction
Siyuan Fang
Motiar Rahaman
Jaya Bharti
Erwin Reisner
Marc Robert
Geoffrey A. Ozin
Yun Hang Hu
Nature Reviews Methods Primers, 3

← 1 2 3 4 5 →