Finite-size scaling for the glass transition: The role of a static length scale

被引:26
|
作者
Karmakar, Smarajit [1 ]
Procaccia, Itamar [2 ]
机构
[1] Univ Roma La Sapienza, Dept Fis, I-00185 Rome, Italy
[2] Weizmann Inst Sci, Dept Chem Phys, IL-76100 Rehovot, Israel
来源
PHYSICAL REVIEW E | 2012年 / 86卷 / 06期
基金
以色列科学基金会; 欧洲研究理事会;
关键词
POTENTIAL-ENERGY LANDSCAPE; NONLINEAR SUSCEPTIBILITY; DYNAMICS;
D O I
10.1103/PhysRevE.86.061502
中图分类号
O35 [流体力学]; O53 [等离子体物理学];
学科分类号
070204 ; 080103 ; 080704 ;
摘要
Over the past decade, computer simulations have had an increasing role in shedding light on difficult statistical physical phenomena, and in particular on the ubiquitous problem of the glass transition. Here in a wide variety of materials the viscosity of a supercooled liquid increases by many orders of magnitude upon decreasing the temperature over a modest range. A natural concern in these computer simulations is the very small size of the simulated systems compared to experimental ones, raising the issue of how to assess the thermodynamic limit. Here we turn this limitation to our advantage by performing finite size scaling on the system size dependence of the relaxation time for supercooled liquids to emphasize the importance of a growing static length scale in the theory of glass transition. We demonstrate that the static length scale that was discovered by us in Physica A 391, 1001 (2012) fits the bill extremely well, allowing us to provide a finite-size scaling theory for the alpha-relaxation time of the glass transition, including predictions for the thermodynamic limit based on simulations in small systems. DOI: 10.1103/PhysRevE.86.061502
引用
收藏
页数:6
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