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17O NMR study of the triangular lattice antiferromagnet CuCrO2
被引:6
|作者:
Ogloblichev, Vasily V.
[1
,2
,3
]
Smolnikov, Alexey G.
[1
]
Sadykov, Almaz F.
[1
]
Piskunov, Yuri V.
[1
]
Gerashenko, Alexander P.
[1
]
Furukawa, Yuji
[2
,3
]
Kumagai, Ken-ichi
[3
]
Yakubovsky, Andrey Yu.
[4
]
Mikhalev, Konstantin N.
[1
]
Barilo, Sergei N.
[5
]
Shiryaev, Sergei V.
[5
]
Belozerov, Alexander S.
[1
]
机构:
[1] Russian Acad Sci, Ural Branch, MN Mikheev Inst Met Phys, 18 S Kovalevskaya St, Ekaterinburg 620108, Russia
[2] Iowa State Univ, Dept Phys & Astron, Ames Lab, Ames, IA 50011 USA
[3] Hokkaido Univ, Fac Sci, Dept Phys, Sapporo, Hokkaido 0600810, Japan
[4] Kurchatov Inst, Natl Res Ctr, Moscow 123182, Russia
[5] Natl Acad Sci Belarus, Inst Solid State Phys & Semicond, Minsk 220072, BELARUS
基金:
俄罗斯科学基金会;
关键词:
O-17;
NMR;
Electric field gradient;
Frustrated systems;
Helicoidal magnetic structure;
SPIN;
RESONANCE;
D O I:
10.1016/j.jmmm.2018.02.080
中图分类号:
T [工业技术];
学科分类号:
08 ;
摘要:
The single crystalline and powder samples of multiferroic CuCrO2 have been investigated by O-17 NMR techniques in the paramagnetic and magnetically ordered states. The unusual negative hyperfine field on oxygen nuclei, H-hf = -5.2 kOe/mu B, has been determined in paramagnetic state. The O-17 NMR spectrum in ordered state has a shape typical for incommensurate magnetic structure. It can be well described taking into account only dipole fields which are produced by Cr3+- ions with magnetic moment mu = 2.2 mu(B). The parameters of the EFG (electric field gradient) tensor - the quadrupole frequency (upsilon(Q)) and the asymmetry parameter, have been determined. The value of upsilon(Q) increases monotonously with decreasing temperature in the range 90 K > T > 1.5 K. The estimates of the population of the ligands p - orbitals have been obtained. (C) 2018 Elsevier B.V. All rights reserved.
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页码:1 / 9
页数:9
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