Photocatalyst-free visible-light-induced highly selective acylation of purine nucleosides at the C6 position

被引：10
|
作者：
Li, Luohao [1 ]
Zheng, Huiqin [1 ]
Guo, Feixiang [1 ]
Fang, Zehui [2 ]
Sun, Qianqian [1 ]
Li, Jing [1 ]
Gao, Qinghe [1 ]
Zhang, Tao [1 ]
Fang, Lizhen [1 ]
机构：
[1] Xinxiang Med Univ, Sch Pharm, Xinxiang 453003, Henan, Peoples R China
[2] Yanbian Univ, Coll Med, Yanji 133002, Jilin, Peoples R China
来源：
CHEMICAL COMMUNICATIONS | 2023年 / 59卷 / 26期
关键词：
MINISCI-TYPE ALKYLATION; ALIPHATIC-ALDEHYDES; HETEROCYCLES; ROUTE;
D O I：
10.1039/d3cc00906h
中图分类号：
O6 [化学];
学科分类号：
0703 ;
摘要：
A protocol for visible-light-induced C-H acylation selectively at the C6 position of purine nucleosides with aldehydes under photocatalyst-free conditions was established herein. This protocol allows the green, mild, and efficient functionalization of various purine nucleosides with a broad range of alkyl and aryl aldehydes.
引用
收藏
页码：3910 / 3913
页数：4
相关论文
共 50 条
  • [1] Metal- and photocatalyst-free approach to visible-light-induced acylation of quinoxalinones
    Niwetmarin, Worawat
    Saesian, Naiyana
    Saruengkhanphasit, Rungroj
    Eurtivong, Chatchakorn
    Thasana, Nopporn
    Ruchirawat, Somsak
    ORGANIC & BIOMOLECULAR CHEMISTRY, 2024, 22 (29) : 5924 - 5929
  • [2] Visible-Light-Induced Photocatalyst-Free Radical Trifluoromethylation
    Li, Yufei
    Liang, Xin
    Niu, Kaikai
    Gu, Jun
    Liu, Fang
    Xia, Qing
    Wang, Qingmin
    Zhang, Weihua
    ORGANIC LETTERS, 2022, 24 (32) : 5918 - 5923
  • [3] Visible-light-induced photocatalyst-free dearomative amidation of phenol derivatives
    Wu, Lingang
    Sun, Lei
    Liu, Wanxing
    Cui, Jichun
    Xie, Lei
    TETRAHEDRON LETTERS, 2023, 128
  • [4] A visible-light-induced photocatalyst-free approach for C-3 dicarbonyl coumarin production
    Xi, Jinhu
    Wu, Xinjie
    Huang, Mengmeng
    Kim, Jung Keun
    Zhang, Jianye
    Li, Yabo
    Wu, Yangjie
    CHEMICAL COMMUNICATIONS, 2021, 57 (59) : 7308 - 7311
  • [5] Visible-light-induced photocatalyst-free C-3 functionalization of indoles with diethyl bromomalonate
    Gu, Guangmiao
    Huang, Mengmeng
    Kim, Jung Keun
    Zhang, Jianye
    Li, Yabo
    Wu, Yangjie
    GREEN CHEMISTRY, 2020, 22 (08) : 2543 - 2548
  • [6] External Photocatalyst-Free Visible-Light-Induced C3-Acylation of Quinoxalin-2(1H)-ones
    Shi, Jianwei
    Wei, Wei
    CHINESE JOURNAL OF ORGANIC CHEMISTRY, 2020, 40 (07) : 2170 - 2172
  • [7] Visible-Light-Induced Metal-/Photocatalyst-Free C-H Bond Imidation of Arenes
    Kuribara, Takahito
    Nakajima, Masaya
    Nemoto, Tetsuhiro
    ORGANIC LETTERS, 2020, 22 (06) : 2235 - 2239
  • [8] Visible-light-promoted photocatalyst-free alkylation and acylation of benzothiazoles
    Jiang, Pengxing
    Liu, Li
    Tan, Jiajing
    Du, Hongguang
    ORGANIC & BIOMOLECULAR CHEMISTRY, 2021, 19 (20) : 4487 - 4491
  • [9] Direct C-H sulfenylation of quinoxalinones with thiols under visible-light-induced photocatalyst-free conditions
    Teng, Qing-Hu
    Yao, Yan
    Wei, Wen-Xiu
    Tang, Hai-Tao
    Li, Jia-Rong
    Pan, Ying-Ming
    GREEN CHEMISTRY, 2019, 21 (23) : 6241 - 6245
  • [10] Visible-Light-Induced Catalytic Selective Halogenation with Photocatalyst
    Luu, Truong Giang
    Jung, Yongju
    Kim, Hee-Kwon
    MOLECULES, 2021, 26 (23):
12345