Mesoporous single-crystal-based TiO2 microspheres decorated by carbon nitride for obviously improved photocatalytic performance and recyclability

被引:0
|
作者
Li, Chen [1 ]
Shen, Shitai [2 ]
Niu, Jinan [1 ]
Reka, Arianit A. [3 ]
Feng, Peizhong [1 ]
Garcia, Hermenegildo [4 ]
机构
[1] China Univ Min & Technol, Sch Mat Sci & Phys, Xuzhou 221116, Peoples R China
[2] Xuzhou Construction Machinery Grp Co Ltd, Sci Technol & Qual Dept, Xuzhou 221004, Peoples R China
[3] Univ Tetova, Fac Nat Sci & Math, Tetovo 1200, North Macedonia
[4] Univ Politecn Valencia, Inst Tecnol Quim CSIC UPV, Valencia 46022, Spain
关键词
Porous single crystals; Z -scheme heterojunction; Photocatalysis; TiO2; DEGRADATION; C3N4;
D O I
10.1016/j.inoche.2023.110524
中图分类号
O61 [无机化学];
学科分类号
070301 ; 081704 ;
摘要
A novel porous TiO2 (PT) with mesoporous single-crystal-based microsphere morphology has been synthesized by a hard-template method and then decorated by graphitic carbon nitride (g-C3N4, CN) nanosheets. The prepared composites (CN/PT) exhibit improved photocatalytic activity in degradation of methylene blue (MB) compared to nonporous bulk TiO2 (BT), PT and g-C3N4, and much better recyclability than commercial P25 TiO2. The enhancement of photocatalytic activity of composites can be attributed to the increased active sites on PT surfaces, and the Z-scheme heterojunction promoting charge separation of photogenerated carriers.
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页数:4
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