Mesoporous single-crystal-based TiO2 microspheres decorated by carbon nitride for obviously improved photocatalytic performance and recyclability

被引:0
|
作者
Li, Chen [1 ]
Shen, Shitai [2 ]
Niu, Jinan [1 ]
Reka, Arianit A. [3 ]
Feng, Peizhong [1 ]
Garcia, Hermenegildo [4 ]
机构
[1] China Univ Min & Technol, Sch Mat Sci & Phys, Xuzhou 221116, Peoples R China
[2] Xuzhou Construction Machinery Grp Co Ltd, Sci Technol & Qual Dept, Xuzhou 221004, Peoples R China
[3] Univ Tetova, Fac Nat Sci & Math, Tetovo 1200, North Macedonia
[4] Univ Politecn Valencia, Inst Tecnol Quim CSIC UPV, Valencia 46022, Spain
关键词
Porous single crystals; Z -scheme heterojunction; Photocatalysis; TiO2; DEGRADATION; C3N4;
D O I
10.1016/j.inoche.2023.110524
中图分类号
O61 [无机化学];
学科分类号
070301 ; 081704 ;
摘要
A novel porous TiO2 (PT) with mesoporous single-crystal-based microsphere morphology has been synthesized by a hard-template method and then decorated by graphitic carbon nitride (g-C3N4, CN) nanosheets. The prepared composites (CN/PT) exhibit improved photocatalytic activity in degradation of methylene blue (MB) compared to nonporous bulk TiO2 (BT), PT and g-C3N4, and much better recyclability than commercial P25 TiO2. The enhancement of photocatalytic activity of composites can be attributed to the increased active sites on PT surfaces, and the Z-scheme heterojunction promoting charge separation of photogenerated carriers.
引用
收藏
页数:4
相关论文
共 50 条
  • [21] Hierarchical mesoporous TiO2 microspheres for the enhanced photocatalytic oxidation of sulfonamides and their mechanism
    Guo, Changsheng
    Xu, Jian
    Zhang, Yuan
    He, Yan
    RSC ADVANCES, 2012, 2 (11) : 4720 - 4727
  • [22] Hollow mesoporous TiO2 microspheres for enhanced photocatalytic degradation of acetaminophen in water
    Lin, Chin Jung
    Yang, Wen-Ta
    Chou, Chen-Yi
    Liou, Sofia Ya Hsuan
    CHEMOSPHERE, 2016, 152 : 490 - 495
  • [23] N-Cdots-decorated TiO2(B)/anatase microspheres with high photocatalytic performance in visible light
    Song, Tong
    Zhang, Xiao
    Wei, Yan
    Yang, Ping
    INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2019, 44 (59) : 31129 - 31140
  • [24] Enhanced photocatalytic activity of a mesoporous TiO2 aerogel decorated onto three-dimensional carbon foam
    Parale, Vinayak G.
    Kim, Taehee
    Phadtare, Varsha D.
    Yadav, Hemraj M.
    Park, Hyung-Ho
    JOURNAL OF MOLECULAR LIQUIDS, 2019, 277 : 424 - 433
  • [25] Comparative Study into the Photocatalytic Performance of Mesoporous Films of TiO2
    Rathousky, J.
    Kalousek, V.
    PROCEEDINGS OF THE 6TH EUROPEAN MEETING ON SOLAR CHEMISTRY & PHOTOCATALYSIS: ENVIRONMENTAL APPLICATIONS, 2010, : 55 - 56
  • [26] Anatase TiO2-Decorated Graphitic Carbon Nitride for Photocatalytic Conversion of Carbon Dioxide
    Tseng, I-Hsiang
    Sung, Yu-Min
    Chang, Po-Ya
    Chen, Chin-Yi
    POLYMERS, 2019, 11 (01)
  • [27] Ag2O nanop article-decorated TiO2 nanobelts for improved photocatalytic performance
    He, Haiyan
    Miao, Yanping
    Du, Yingying
    Zhao, Jie
    Liu, Yunshi
    Yang, Ping
    CERAMICS INTERNATIONAL, 2016, 42 (01) : 97 - 102
  • [28] Mesoporous TiO2 microspheres with improved efficiency for photooxidation of volatile organic compounds
    Vitaliy Shvalagin
    Natalia Ermokhina
    Natalia Romanovska
    Roman Barakov
    Petro Manorik
    Vitaliy Sapsay
    Sergey Shcherbakov
    Olga Poddubnaya
    Alexander Puziy
    Research on Chemical Intermediates, 2019, 45 : 4133 - 4148
  • [29] Cu2O decorated carbon-incorporated TiO2 microspheres with enhanced visible light photocatalytic activity
    Fang, Yalin
    Sun, Mingxuan
    Wang, Ying
    Sun, Shanfu
    He, Jia
    MATERIALS RESEARCH BULLETIN, 2016, 74 : 265 - 270
  • [30] Mesoporous TiO2 microspheres with improved efficiency for photooxidation of volatile organic compounds
    Shvalagin, Vitaliy
    Ermokhina, Natalia
    Romanovska, Natalia
    Barakov, Roman
    Manorik, Petro
    Sapsay, Vitaliy
    Shcherbakov, Sergey
    Poddubnaya, Olga
    Puziy, Alexander
    RESEARCH ON CHEMICAL INTERMEDIATES, 2019, 45 (08) : 4133 - 4148