Coherence in Chemistry: Foundations and Frontiers

被引：1

作者：

Schultz, Jonathan D. ^{[1
,2
]}

Yuly, Jonathon L. ^{[3
,4
]}

Arsenault, Eric A. ^{[6
,7
]}

Parker, Kelsey ^{[1
]}

Chowdhury, Sutirtha N. ^{[1
]}

Dani, Reshmi ^{[8
]}

Kundu, Sohang ^{[8
]}

Nuomin, Hanggai ^{[1
]}

Zhang, Zhendian ^{[1
]}

Valdiviezo, Jesus ^{[1
,9
,10
,11
]}

Zhang, Peng ^{[1
]}

Orcutt, Kaydren ^{[6
,12
,13
]}

Jang, Seogjoo J. ^{[14
,15
]}

Fleming, Graham R. ^{[6
]}

Makri, Nancy ^{[8
,16
,18
]}

Ogilvie, Jennifer P. ^{[17
]}

Therien, Michael J. ^{[1
]}

Wasielewski, Michael R. ^{[2
]}

Beratan, David N. ^{[1
,4
,5
]}

机构：

[1] Duke Univ, Dept Chem, Durham, NC 27708 USA

[2] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA

[3] Princeton Univ, Lewis Sigler Inst Integrat Genom, Princeton, NJ 08540 USA

[4] Duke Univ, Dept Phys, Durham, NC 27708 USA

[5] Duke Univ, Dept Biochem, Durham, NC 27710 USA

[6] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA

[7] Columbia Univ, Dept Chem, New York, NY 10027 USA

[8] Univ Illinois, Dept Chem, Urbana, IL 61801 USA

[9] Harvard Med Sch, Dept Biol Chem & Mol Pharmacol, Boston, MA 02115 USA

[10] Dana Farber Canc Inst, Dept Canc Biol, Boston, MA 02215 USA

[11] Pontificia Univ Catolica Peru, Dept Psychol, Secc Quim, San Miguel 15088, Lima, Peru

[12] Lawrence Berkeley Natl Lab, Mol Biophys & Integrated Bioimaging Div, Berkeley, CA 94720 USA

[13] ARS, Bioprod Res Unit, Western Reg Res Ctr, USDA, Albany, CA 94710 USA

[14] CUNY Queens Coll, Dept Chem & Biochem, Queens, NY 11367 USA

[15] CUNY, Grad Ctr, Chem & Phys PhD Programs, New York, NY 10016 USA

[16] Univ Illinois, Dept Phys, Urbana, IL 61801 USA

[17] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA

[18] Univ Illinois, Illinois Quantum Informat Sci & Technol Ctr, Urbana, IL 61801 USA

来源：

CHEMICAL REVIEWS | 2024年 / 124卷 / 21期

基金：

美国国家科学基金会;

关键词：

EXCITATION-ENERGY TRANSFER; 2-DIMENSIONAL ELECTRONIC SPECTROSCOPY; LIGHT-HARVESTING COMPLEX; BACKWARD SEMICLASSICAL DYNAMICS; INITIAL-VALUE REPRESENTATION; POLYMER MOLECULAR-DYNAMICS; QUANTUM MASTER EQUATION; PHOTOSYNTHETIC REACTION CENTERS; DISSIPATIVE 2-LEVEL SYSTEMS; PATH-INTEGRAL CALCULATION;

D O I：

10.1021/acs.chemrev.3c00643

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Coherence refers to correlations in waves. Because matter has a wave-particle nature, it is unsurprising that coherence has deep connections with the most contemporary issues in chemistry research (e.g., energy harvesting, femtosecond spectroscopy, molecular qubits and more). But what does the word "coherence" really mean in the context of molecules and other quantum systems? We provide a review of key concepts, definitions, and methodologies, surrounding coherence phenomena in chemistry, and we describe how the terms "coherence" and "quantum coherence" refer to many different phenomena in chemistry. Moreover, we show how these notions are related to the concept of an interference pattern. Coherence phenomena are indeed complex, and ambiguous definitions may spawn confusion. By describing the many definitions and contexts for coherence in the molecular sciences, we aim to enhance understanding and communication in this broad and active area of chemistry.

引用

页码：11641 / 11766

页数：126

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