Ground-penetrating radar (GPR) is a pivotal noninvasive tool that yields subsurface images critical to archeology, near-surface characterization, geotechnical studies, and disaster response. The antenna central frequency of the GPR system has a significant impact on penetration depth and resolution. Lower antenna frequencies penetrate deeper but at lower resolutions, while higher frequencies offer detailed images at reduced depths. Therefore, improving the resolution of low-frequency radar with increased detection depth is an essential research focus. Inspired by image super-resolution advancements, supervised deep learning methods that rely on strictly paired training data have achieved remarkable success. However, acquiring such paired samples in practical scenarios is often a formidable challenge. To tackle this, we propose a novel resolution enhancement technique through weakly supervised learning, effectively addressing the scarcity of strictly paired samples in real-world situations. We utilize two sets of antennas with different central frequencies to construct our training data, with a low-frequency antenna as input and a high-frequency antenna as the learning target. A cycle-consistent generative adversarial network (Cycle-GAN) is trained to discern the mapping between low-resolution inputs and unpaired high-resolution data. The refined network is then employed to improve low-frequency GPR data resolution. Our work is validated on synthetic and real-world datasets. The proposed method effectively strengthens critical high-frequency details for finer imaging and broadens the frequency bandwidth. Significantly, it enhances resolution without compromising the detection depth of low-resolution GPR data, marking a substantial advancement in subsurface imaging technology.