The Rise of 2D Materials-Based Photoelectrochemical Photodetectors: Progress and Prospect

2D materials have garnered significant research attention due to their unique electrical and optical properties. Various photodetectors (PDs) based on 2D materials have been demonstrated to possess a high photoresponse, achieve specific light detection, and construct flexible devices. Among these, photoelectrochemical-type (PEC) PDs are attracting increasing attention due to their facile fabrication processes, self-powered capability, and high sensitivity. Compared with transitional solid-state PDs based on 2D materials, research on 2D material-based PEC PDs is still in its initial stages but exhibits promising potential for various applications. This paper comprehensively reviews recent advancements in 2D material-based PEC PDs. The 2D materials for PEC PDs are first classified, and then the synthesis methods employed for their fabrication are briefly summarized. Later, the performance and performance optimization strategies of various 2D material-based PEC PDs are discussed. Finally, the challenges and opportunities for developing high-performance 2D material-based PEC PDs are highlighted. Providing a comprehensive review conducted on 2D material-based photoelectrochemical photodetectors (PEC PDs). This review introduces the basic theory of PEC PDs and systematically classifies 2D materials applied in PEC PDs and their preparation methods. In addition, the performance and optimization strategies of 2D material-based PEC PDs are evaluated and summarized, elaborating strategies and prospects for developing high-performance PEC PDs. image