PUMP-PROBE SPECTROSCOPY AND EXCITON DYNAMICS OF J-AGGREGATES AT HIGH PUMP INTENSITIES

被引：65
|
作者：
JOHNSON, AE [1 ]
KUMAZAKI, S [1 ]
YOSHIHARA, K [1 ]
机构：
[1] INST MOLEC SCI,OKAZAKI,AICHI 444,JAPAN
来源：
CHEMICAL PHYSICS LETTERS | 1993年 / 211卷 / 06期
关键词：
D O I：
10.1016/0009-2614(93)80135-C
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
We have measured the picosecond pump-probe spectra of BIC J aggregates using a spectral continuum for the probe. The excitation pulses were intense (10(15)-2 X 10(16) photons/cm2) and created many excitons per aggregate. The observed dynamics are intensity dependent and reflect exciton-exciton annihilation processes. In addition, the zero-time spectrum is also intensity dependent, probably due to a reduction of k space at high exciton concentrations.
引用
收藏
页码：511 / 515
页数：5
相关论文
共 50 条
  • [31] Pump built-in Hamiltonian method for pump-probe spectroscopy
    Inoue, JI
    Shimizu, A
    JOURNAL OF THE PHYSICAL SOCIETY OF JAPAN, 1999, 68 (08) : 2534 - 2537
  • [32] Pump-probe spectra of linear molecular aggregates: Effect of exciton-exciton interaction and higher molecular levels
    Juzeliunas, G
    Reineker, P
    JOURNAL OF CHEMICAL PHYSICS, 1998, 109 (16): : 6916 - 6928
  • [33] Influence of exciton-exciton interaction and of higher molecular levels on the pump-probe spectra of linear molecular aggregates
    Juzeliunas, G
    Reineker, P
    PROCEEDINGS OF THE THIRD INTERNATIONAL CONFERENCE ON EXCITONIC PROCESSES IN CONDENSED MATTER - EXCON '98, 1998, 98 (25): : 105 - 110
  • [34] Third-order pump-probe spectroscopy applied to molecular dimers: characterization of relaxation dynamics and exciton-exciton annihilation
    Glaab, Fabian
    Suess, Jasmin
    Engel, Volker
    PHYSICAL CHEMISTRY CHEMICAL PHYSICS, 2022, 24 (41) : 25316 - 25326
  • [35] Polarization-resolved pump-probe spectroscopy with high harmonics
    Mairesse, Y.
    Haessler, S.
    Fabre, B.
    Higuet, J.
    Boutu, W.
    Breger, P.
    Constant, E.
    Descamps, D.
    Mevel, E.
    Petit, S.
    Salieres, P.
    NEW JOURNAL OF PHYSICS, 2008, 10
  • [36] ULTRAFAST SPECTROSCOPY OF PICBR J-AGGREGATES - THE DYNAMICS OF LARGE COHERENCE LENGTH EXCITON
    KOBAYASHI, S
    SASAKI, F
    JOURNAL OF LUMINESCENCE, 1994, 58 (1-6) : 113 - 116
  • [37] Pump-probe spectroscopy study of ultrafast temperature dynamics in nanoporous gold
    Ortolani, Michele
    Mancini, Andrea
    Budweg, Arne
    Garoli, Denis
    Brida, Daniele
    de Angelis, Francesco
    PHYSICAL REVIEW B, 2019, 99 (03)
  • [38] Simulation of ultrafast dynamics and pump-probe spectroscopy using classical trajectories
    Li, ZM
    Fang, JY
    Martens, CC
    JOURNAL OF CHEMICAL PHYSICS, 1996, 104 (18): : 6919 - 6929
  • [39] Femtosecond pump-probe spectroscopy investigation of carrier dynamics in GaAlAs photocathods
    Feng, Aiming
    Yin, Lin
    Zhang, Shuqin
    Chen, Liang
    Qian, Yunshen
    Jani, Hemang
    Duan, Lingze
    OPTIK, 2019, 179 : 336 - 340
  • [40] Excited state dynamics of oligothiophenes studied by transient pump-probe spectroscopy
    Lanzani, G
    Cerullo, G
    Stagira, S
    De Silvestri, S
    JOURNAL OF PHOTOCHEMISTRY AND PHOTOBIOLOGY A-CHEMISTRY, 2001, 144 (01) : 13 - 19
12345