ON THE INFLUENCE OF COHERENT INELASTIC RESONANCE SCATTERING ON THE MOSSBAUER ABSORPTION-SPECTRA

被引:2
|
作者
BELYAKOV, VA
机构
[1] All-Union Surface and Vacuum Research Centre, Moscow
来源
HYPERFINE INTERACTIONS | 1991年 / 67卷 / 1-4期
关键词
D O I
10.1007/BF02398212
中图分类号
O64 [物理化学(理论化学)、化学物理学]; O56 [分子物理学、原子物理学];
学科分类号
070203 ; 070304 ; 081704 ; 1406 ;
摘要
It is shown that an unusual angular distribution in coherent inelastic Mossbauer scattering (MCIS) manifests itself in Mossbauer absorption spectra (MAS). This is due to the fact that MCIS connected with the phonon assisted processes is concentrated in the direction of the incident Mossbauer beam propagation. The manifestation of MCIS in MAS in the case of MAS hyperfine splitting is analyzed. The effect reveals itself in the ratios of hyperfine line intensities in MAS due to the fact that the MCIS cross-section is different for different MAS hyperfine lines. In particular, for the case of thick nuclear resonance absorber the dips in MAS are different for the different hyperfine lines. (Usually it is assumed that for thick absorber the amplitudes of the dips are the same for all lines.) The general expressions for the intensity ratios for different MAS hyperfine lines which take into account MCIS are given in the case of hyperfine magnetic splitting. Estimates show that the corrections to the conventionally assumed ratios of line intensities in MAS are usually not large but quite measureable. However in the favorable cases (isotopes with low values of internal conversion coefficients) they can be as large as ten percent.
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页码:633 / 639
页数:7
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