SPECTRAL DIFFUSION IN AN AMORPHOUS POLYMER PROBED BY SINGLE-MOLECULE SPECTROSCOPY

被引：55
|
作者：
TITTEL, J
KETTNER, R
BASCHE, T
BRAUCHLE, C
QUANTE, H
MULLEN, K
机构：
[1] UNIV MUNICH,INST PHYS CHEM,D-80333 MUNICH,GERMANY
[2] MAX PLANCK INST POLYMER RES,D-55021 MAINZ,GERMANY
来源：
JOURNAL OF LUMINESCENCE | 1995年 / 64卷 / 1-6期
关键词：
D O I：
10.1016/0022-2313(95)00002-8
中图分类号：
O43 [光学];
学科分类号：
070207 ; 0803 ;
摘要：
We investigated the spectra of single tetra-tert-butylterrylene (TBT) molecules in the amorphous matrix poly(isobutylene) (PIB). The distribution of line widths of TET in PIB was measured and compared to that of TBT in poly(ethylene). The fluorescence intensity autocorrelation function as well as the two-point frequency autocorrelation function were determined for different single TBT molecules. Logarithmic-like decays of the fluorescence autocorrelation function could be reproduced by assuming a 1/R fluctuation rate distribution for the two-level-tunnelling systems.
引用
收藏
页码：1 / 11
页数：11
相关论文
共 50 条
  • [1] On the role of spectral diffusion in single-molecule spectroscopy
    Palm, VV
    Rebane, KK
    Zabrodskii, A
    [J]. PHYSICS OF THE SOLID STATE, 2000, 42 (03) : 477 - 480
  • [2] On the role of spectral diffusion in single-molecule spectroscopy
    Palm, V
    Rebane, K
    [J]. JOURNAL OF LUMINESCENCE, 2000, 86 (3-4) : 207 - 209
  • [3] On the role of spectral diffusion in single-molecule spectroscopy
    V. V. Palm
    K. K. Rebane
    A. Zabrodskii
    [J]. Physics of the Solid State, 2000, 42 : 477 - 480
  • [4] Determination of the spectral diffusion kernel of a protein by single-molecule spectroscopy
    Baier, Juergen
    Richter, Martin F.
    Cogdell, Richard J.
    Oellerich, Silke
    Kohler, Juergen
    [J]. PHYSICAL REVIEW LETTERS, 2008, 100 (01)
  • [5] Single-Molecule Spectroscopy on a Ladder-Type Conjugated Polymer: Electron-Phonon Coupling and Spectral Diffusion
    Hildner, Richard
    Winterling, Laura
    Lemmer, Ulrich
    Scherf, Ullrich
    Koehler, Juergen
    [J]. CHEMPHYSCHEM, 2009, 10 (14) : 2524 - 2534
  • [6] Correlation of emission intensity and spectral diffusion in room temperature single-molecule spectroscopy
    Stracke, F
    Blum, C
    Becker, S
    Müllen, K
    Meixner, AJ
    [J]. CHEMPHYSCHEM, 2005, 6 (07) : 1242 - 1246
  • [7] SPECTRAL DIFFUSION OF SINGLE-MOLECULE LINES IN POLYMERS
    FLEURY, L
    BROWN, R
    BERNARD, J
    ORRIT, M
    [J]. LASER PHYSICS, 1995, 5 (03) : 648 - 651
  • [8] Memory and spectral diffusion in single-molecule emission
    Wustholz, Kristin L.
    Bott, Eric D.
    Kahr, Bart
    Reid, Philip J.
    [J]. JOURNAL OF PHYSICAL CHEMISTRY C, 2008, 112 (21): : 7877 - 7885
  • [9] Single-molecule tracking of polymer surface diffusion
    20140617290006
    [J]. Schwartz, D.K. (daniel.schwartz@colorado.edu), 1600, American Chemical Society (136):
  • [10] Single-Molecule Tracking of Polymer Surface Diffusion
    Skaug, Michael J.
    Mabry, Joshua N.
    Schwartz, Daniel K.
    [J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2014, 136 (04) : 1327 - 1332
12345