Observation of an antiferromagnetic quantum critical point in high-purity LaNiO3

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作者
Changjiang Liu
Vincent F. C. Humbert
Terence M. Bretz-Sullivan
Gensheng Wang
Deshun Hong
Friederike Wrobel
Jianjie Zhang
Jason D. Hoffman
John E. Pearson
J. Samuel Jiang
Clarence Chang
Alexey Suslov
Nadya Mason
M. R. Norman
Anand Bhattacharya
机构
[1] Argonne National Laboratory,Materials Science Division
[2] University of Illinois at Urbana-Champaign,Department of Physics
[3] Argonne National Laboratory,High Energy Physics Division
[4] Harvard University,Department of Physics
[5] National High Magnetic Field Laboratory,undefined
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摘要
Amongst the rare-earth perovskite nickelates, LaNiO3 (LNO) is an exception. While the former have insulating and antiferromagnetic ground states, LNO remains metallic and non-magnetic down to the lowest temperatures. It is believed that LNO is a strange metal, on the verge of an antiferromagnetic instability. Our work suggests that LNO is a quantum critical metal, close to an antiferromagnetic quantum critical point (QCP). The QCP behavior in LNO is manifested in epitaxial thin films with unprecedented high purities. We find that the temperature and magnetic field dependences of the resistivity of LNO at low temperatures are consistent with scatterings of charge carriers from weak disorder and quantum fluctuations of an antiferromagnetic nature. Furthermore, we find that the introduction of a small concentration of magnetic impurities qualitatively changes the magnetotransport properties of LNO, resembling that found in some heavy-fermion Kondo lattice systems in the vicinity of an antiferromagnetic QCP.
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