Perturbations in stratospheric aerosol evolution due to the water-rich plume of the 2022 Hunga-Tonga eruption

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作者
Yunqian Zhu
Charles G. Bardeen
Simone Tilmes
Michael J. Mills
Xinyue Wang
V. Lynn Harvey
Ghassan Taha
Douglas Kinnison
Robert W. Portmann
Pengfei Yu
Karen H. Rosenlof
Melody Avery
Corinna Kloss
Can Li
Anne S. Glanville
Luis Millán
Terry Deshler
Nickolay Krotkov
Owen B. Toon
机构
[1] National Center for Atmospheric Research,Atmospheric Chemistry Observations and Modeling Laboratory
[2] University of Colorado Boulder,Laboratory for Atmospheric and Space Physics
[3] University of Colorado Cooperative Institute for Research in Environmental Sciences (CIRES) at the NOAA Chemical Sciences Laboratory,GESTAR II
[4] Morgan State University,Goddard Space Flight Center
[5] National Aeronautics and Space Administration,Chemical Sciences Laboratory
[6] National Oceanic and Atmospheric Administration,Institute for Environmental and Climate Research
[7] Jinan University,Laboratoire de Physique et Chimie de l’Environnement et de l’Espace
[8] NASA Langley Research Center,Earth System Science Interdisciplinary Center
[9] CNRS UMR 7328,Jet Propulsion Laboratory
[10] Université d’Orléans,Department of Atmospheric and Oceanic Sciences
[11] University of Maryland,undefined
[12] California Institute of Technology,undefined
[13] University of Colorado Boulder,undefined
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摘要
The January 2022 Hunga Tonga-Hunga Ha’apai volcanic eruption injected a relatively small amount of sulfur dioxide, but significantly more water into the stratosphere than previously seen in the modern satellite record. Here we show that the large amount of water resulted in large perturbations to stratospheric aerosol evolution. Our climate model simulation reproduces the observed enhanced water vapor at pressure levels ~30 hPa for three months. Compared with a simulation without a water injection, this additional source of water vapor increases hydroxide, which halves the sulfur dioxide lifetime. Subsequent coagulation creates larger sulfate particles that double the stratospheric aerosol optical depth. A seasonal forecast of volcanic plume transport in the southern hemisphere indicates this eruption will greatly enhance the aerosol surface area and water vapor near the polar vortex until at least October 2022, suggesting that there will continue to be an impact of this eruption on the climate system.
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