Bright single photon emitters with enhanced quantum efficiency in a two-dimensional semiconductor coupled with dielectric nano-antennas

被引:0
|
作者
Luca Sortino
Panaiot G. Zotev
Catherine L. Phillips
Alistair J. Brash
Javier Cambiasso
Elena Marensi
A. Mark Fox
Stefan A. Maier
Riccardo Sapienza
Alexander I. Tartakovskii
机构
[1] University of Sheffield,Department of Physics and Astronomy
[2] Ludwig-Maximilians-Universität München,Chair in Hybrid Nanosystems, Nanoinstitute Munich, Faculty of Physics
[3] Imperial College London,The Blackett Laboratory, Department of Physics
[4] Am Campus 1,IST Austria
来源
关键词
D O I
暂无
中图分类号
学科分类号
摘要
Single photon emitters in atomically-thin semiconductors can be deterministically positioned using strain induced by underlying nano-structures. Here, we couple monolayer WSe2 to high-refractive-index gallium phosphide dielectric nano-antennas providing both optical enhancement and monolayer deformation. For single photon emitters formed on such nano-antennas, we find very low (femto-Joule) saturation pulse energies and up to 104 times brighter photoluminescence than in WSe2 placed on low-refractive-index SiO2 pillars. We show that the key to these observations is the increase on average by a factor of 5 of the quantum efficiency of the emitters coupled to the nano-antennas. This further allows us to gain new insights into their photoluminescence dynamics, revealing the roles of the dark exciton reservoir and Auger processes. We also find that the coherence time of such emitters is limited by intrinsic dephasing processes. Our work establishes dielectric nano-antennas as a platform for high-efficiency quantum light generation in monolayer semiconductors.
引用
收藏
相关论文
共 50 条
  • [21] Quantum chaos in nano-sized billiards in layered two-dimensional semiconductor structures
    Berggren, KF
    Ji, ZL
    CHAOS, 1996, 6 (04) : 543 - 553
  • [22] Modulating the single-photon transport periodically with two emitters in two one-dimensional coupled cavity arrays
    Shi, Yun-Xia
    Tan, Lei
    Liang, Jun-Jie
    Li, Qing
    Ma, Jin-Lou
    OPTICS COMMUNICATIONS, 2019, 431 : 73 - 80
  • [23] Resonance Fluorescence from Waveguide-Coupled, Strain-Localized, Two-Dimensional Quantum Emitters
    Errando-Herranz, Carlos
    Schoell, Eva
    Picard, Raphael
    Laini, Micaela
    Gyger, Samuel
    Elshaari, Ali W.
    Branny, Art
    Wennberg, Ulrika
    Barbat, Sebastien
    Renaud, Thibaut
    Sartison, Marc
    Brotons-Gisbert, Mauro
    Bonato, Cristian
    Gerardot, Brian D.
    Zwiller, Val
    Joens, Klaus D.
    ACS PHOTONICS, 2021, 8 (04) : 1069 - 1076
  • [24] Dielectric Function of Two-Dimensional Nanostructure, Including Single Layer Quantum Well
    Tovstyuk, C. C.
    ACTA PHYSICA POLONICA A, 2022, 141 (04) : 341 - 344
  • [25] Microcavity enhanced single photon emission from two-dimensional WSe2
    Flatten, L. C.
    Weng, L.
    Branny, A.
    Johnson, S.
    Dolan, P. R.
    Trichet, A. A. P.
    Gerardot, B. D.
    Smith, J. M.
    APPLIED PHYSICS LETTERS, 2018, 112 (19)
  • [26] Rapid Optical Spin Initialization of a Quantum Dot in the Voigt Geometry Coupled to a Two-Dimensional Semiconductor
    Stefanatos, Dionisis
    Karanikolas, Vasilios
    Iliopoulos, Nikos
    Paspalakis, Emmanuel
    APPLIED SCIENCES-BASEL, 2020, 10 (03):
  • [27] Single-exciton trapping in an electrostatically defined two-dimensional semiconductor quantum dot
    Shanks, Daniel N.
    Mahdikhanysarvejahany, Fateme
    Koehler, Michael R.
    Mandrus, David G.
    Taniguchi, Takashi
    Watanabe, Kenji
    LeRoy, Brian J.
    Schaibley, John R.
    PHYSICAL REVIEW B, 2022, 106 (20)
  • [28] Computational search for efficient single-photon emitters among the substitutional doping defects in two-dimensional GaSe
    Stolbov, Sergey
    Zahir, Rumana
    PHYSICA E-LOW-DIMENSIONAL SYSTEMS & NANOSTRUCTURES, 2023, 153
  • [29] Photon-Phonon-Enhanced Infrared Rectification in a Two-Dimensional Nanoantenna-Coupled Tunnel Diode
    Kadlec, Emil A.
    Jarecki, Robert L.
    Starbuck, Andrew
    Peters, David W.
    Davids, Paul S.
    PHYSICAL REVIEW APPLIED, 2016, 6 (06):
  • [30] Enhanced light extraction efficiency for glass scintillator coupled with two-dimensional photonic crystal structure
    Zhu, Zhichao
    Liu, Bo
    Cheng, Chuanwei
    Yi, Yasha
    Guo, Wenli
    Huang, Shiming
    Chen, Hong
    Gu, Mu
    Ni, Chen
    Liu, Xiaolin
    OPTICAL MATERIALS, 2013, 35 (12) : 2343 - 2346