Single-Atom Pt as Co-Catalyst for Enhanced Photocatalytic H2 Evolution

被引：1193

作者：

Li, Xiaogang ^{[1
]}

Bi, Wentuan ^{[1
]}

Zhang, Lei ^{[2
]}

Tao, Shi ^{[3
]}

Chu, Wangsheng ^{[3
]}

Zhang, Qun ^{[2
]}

Luo, Yi ^{[2
]}

Wu, Changzheng ^{[1
]}

Xie, Yi ^{[1
]}

机构：

[1] Univ Sci & Technol China, CAS Ctr Excellence Nanosci, CAS Key Lab Mech Behav & Design Mat, Hefei Natl Lab Phys Sci Microscale,Collaborat Inn, Hefei 230026, Anhui, Peoples R China

[2] Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Synerget Innovat Ctr Quantum Informat & Quantum P, Hefei 230026, Anhui, Peoples R China

[3] Univ Sci & Technol China, Natl Synchrotron Radiat Lab, Hefei 230026, Anhui, Peoples R China

来源：

ADVANCED MATERIALS | 2016年 / 28卷 / 12期

基金：

中国国家自然科学基金;

关键词：

GRAPHITIC CARBON NITRIDE; HYDROGEN-PRODUCTION; WATER; PLATINUM; NANOPARTICLES; CONVERSION; METHANE; OXIDE; UREA;

D O I：

10.1002/adma.201505281

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Isolated single-atom platinum (Pt) embedded in the sub-nanoporosity of 2D g-C3N4 as a new form of co-catalyst is reported. The highly stable single-atom co-catalyst maximizes the atom efficiency and alters the surface trap states of g-C3N4, leading to significantly enhanced photocatalytic H-2 evolution activity, 8.6 times higher than that of Pt nanoparticles and up to 50 times that for bare g-C3N4.

引用

页码：2427 / 2431

页数：5

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