Silicon Nanoantenna Mix Arrays for a Trifecta of Quantum Emitter Enhancements

被引:30
|
作者
Dong, Zhaogang [1 ]
Gorelik, Sergey [1 ]
Paniagua-Dominguez, Ramon [1 ]
Yik, Johnathan [2 ]
Ho, Jinfa [1 ]
Tjiptoharsono, Febiana [1 ]
Lassalle, Emmanuel [1 ]
Rezaei, Soroosh Daqiqeh [3 ]
Neo, Darren C. J. [1 ]
Bai, Ping [2 ]
Kuznetsov, Arseniy, I [1 ]
Yang, Joel K. W. [1 ,3 ]
机构
[1] ASTAR, Inst Mat Res & Engn, Innovis, Singapore 138634, Singapore
[2] ASTAR, Inst High Performance Comp, Connexis, Singapore 138632, Singapore
[3] Singapore Univ Technol & Design, Singapore 487372, Singapore
关键词
Dielectric nanoantenna; Si nanoantenna; Mie resonance; Directional emission; Purcell factor; 2ND-HARMONIC GENERATION; RHODAMINE; 6G; RESONANCES; COLOR; METASURFACE; EMISSION; NANOSTRUCTURES; NANOPARTICLES; FLUORESCENCE; ANTENNAS;
D O I
10.1021/acs.nanolett.1c01570
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Dielectric nanostructures have demonstrated optical antenna effects due to Mie resonances. Previous work has exhibited enhancements in absorption, emission rates and directionality with practical limitations. In this paper, we present a Si mix antenna array to achieve a trifecta enhancement of similar to 1200-fold with a Purcell factor of similar to 47. The antenna design incorporates similar to 10 nm gaps, within which fluorescent molecules strongly absorb the pump laser energy through a resonant mode. In the emission process, the antenna array increases the radiative decay rates of the fluorescence molecules via a Purcell effect and provides directional emission through a separate mode. This work could lead to novel CMOS-compatible platforms to enhance fluorescence for biological and chemical applications.
引用
收藏
页码:4853 / 4860
页数:8
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