Decomposition of ammonia and hydrogen sulfide in simulated sludge drying waste gas by a novel non-thermal plasma

被引:24
|
作者
Lu, Shengyong [1 ]
Chen, Lu [1 ]
Huang, Qunxing [1 ]
Yang, Liqin [1 ]
Du, Changming [1 ]
Li, Xiaodong [1 ]
Yan, Jianhua [1 ]
机构
[1] Zhejiang Univ, State Key Lab Clean Energy Utilizat, Hangzhou 310027, Zhejiang, Peoples R China
基金
中国国家自然科学基金;
关键词
Plasma; Gliding arc; Ammonia; Hydrogen sulfide; Sludge drying waste gas; PULSE CORONA REACTOR; DISCHARGE PLASMA; EMISSION CHARACTERISTICS; REMOVAL; ARC; VOCS; NH3; H2S;
D O I
10.1016/j.chemosphere.2014.10.036
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
To efficiently clean NH3 and H2S contained in municipal sewage sludge drying waste gas, experiments were conducted with a novel gliding arc discharge plasma reactor. Important parameters including applied voltage and gas velocity which can strongly influence the removal efficiency, energy cost and by-products yields were investigated. Maximum removal efficiencies were all obtained at the applied voltage of 11 kV and gas velocity of 4.72 m s(-1). When NH3 and H2S were treated together, the total energy cost decreased by 38%. NO and SO2 were observed as main decomposition by-products, and the presence of NH3 may inhibit the production of SO2 whose yield decreased from 223.8 to 27.8 mg m(-3). Tests performed on lab scale reactor showed that gliding arc discharge is efficient in decreasing the NH3 and H2S concentrations, and experiments will also be conducted on a larger scale reactor in the future. (C) 2014 Elsevier Ltd. All rights reserved.
引用
收藏
页码:781 / 785
页数:5
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