Role of spin fluctuations in the conductivity of CrO2

We present a time-resolved terahertz spectroscopic study of the half-metallic ferromagnet CrO2. The ultrafast conductivity dynamics excited by an optical pump displays very short (several picoseconds) and a very long (several hundred picoseconds) characteristic time scales. We attribute the former to the electron-phonon relaxation and the latter to the spin-lattice relaxation. We use this distinction to quantify the relative contribution of the scattering by spin fluctuations to the resistivity of CrO2: We find that they contribute less than one half of all scattering events below room temperature. This contribution rises to similar to 70% as the temperature approaches T-C = 390 K. The small effect of spin fluctuations on the resistivity is unexpected in light of the proposed double-exchange nature of the electronic and magnetic properties of CrO2.