High resolution core level spectroscopy of hydrogen-terminated (100) diamond

被引：17

作者：

Schenk, A. K. ^{[1
]}

Rietwyk, K. J. ^{[2
]}

Tadich, A. ^{[1
,3
]}

Stacey, A. ^{[4
]}

Ley, L. ^{[1
,5
]}

Pakes, C. I. ^{[1
]}

机构：

[1] La Trobe Univ, La Trobe Inst Mol Sci, Dept Chem & Phys, Bundoora, Vic 3086, Australia

[2] Bar Ilan Univ, Ctr Nanotechnol & Adv Mat, Dept Chem, IL-5290002 Ramat Gan, Israel

[3] Australian Synchrotron, 800 Blackburn Rd, Clayton, Vic 3168, Australia

[4] Univ Melbourne, Ctr Quantum Computat & Commun Technol, Sch Phys, Melbourne, Vic 3010, Australia

[5] Univ Erlangen Nurnberg, Inst Tech Phys, Staudtstr 1, D-91058 Erlangen, Germany

来源：

JOURNAL OF PHYSICS-CONDENSED MATTER | 2016年 / 28卷 / 30期

基金：

澳大利亚研究理事会;

关键词：

photoelectron spectroscopy; hydrogen-terminated diamond; diamond (100) surface; X-RAY PHOTOEMISSION; ABSORPTION FINE-STRUCTURE; SINGLE-CRYSTAL; SURFACE; SPECTRA; ORIGIN;

D O I：

10.1088/0953-8984/28/30/305001

中图分类号：

O469 [凝聚态物理学];

学科分类号：

070205 ;

摘要：

Synchrotron-based photoelectron spectroscopy experiments are presented that address a long standing inconsistency in the treatment of the C1s core level of hydrogen terminated (1 0 0) diamond. Through a comparison of surface and bulk sensitive measurements we show that there is a surface related core level component to lower binding energy of the bulk diamond component; this component has a chemical shift of -0.16 +/- 0.05 eV which has been attributed to carbon atoms which are part of the hydrogen termination. Additionally, our results indicate that the asymmetry of the hydrogen terminated (1 0 0) diamond C1s core level is an intrinsic aspect of the bulk diamond peak which we have attributed to sub-surface carbon layers.

引用

页数：12

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