Multifunctional carbon-based metal-free catalysts for advanced energy conversion and storage

被引：77
|
作者：
Hu, Chuangang [1 ]
Dai, Quanbin [2 ]
Dai, Liming [1 ]
机构：
[1] Univ New South Wales, Australian Carbon Mat Ctr A CMC, Sch Chem Engn, Sydney, NSW 2052, Australia
[2] Case Western Reserve Univ, Dept Macromol Sci & Engn, 10900 Euclid Ave, Cleveland, OH 44106 USA
来源：
CELL REPORTS PHYSICAL SCIENCE | 2021年 / 2卷 / 02期
基金：
澳大利亚研究理事会;
关键词：
OXYGEN REDUCTION REACTION; REDUCED GRAPHENE OXIDE; DOPED HOLEY GRAPHENE; ACTIVE-SITES; FREE ELECTROCATALYSTS; HIGHLY-EFFICIENT; POROUS CARBON; DEFECT-RICH; BIFUNCTIONAL ELECTROCATALYST; LI-CO2; BATTERIES;
D O I：
10.1016/j.xcrp.2021.100328
中图分类号：
O6 [化学];
学科分类号：
0703 ;
摘要：
Recent advances in research and development of carbon-based metal-free catalysts (C-MFCs) have opened up new research areas for multifunctional electrocatalysis of the oxygen reduction reaction (ORR) in fuel cells, the ORR and oxygen evolution reaction (OER) in metal-air batteries, and the OER and hydrogen evolution reaction (HER) for overall water splitting. New fundamentals governing multifunctional metal-free carbon electrocatalysis were discovered, and recent breakthroughs in this emerging field have enabled C-MFCs to be used as metal-free multifunctional electrocatalysts for various energy-related reactions even beyond the ORR, OER, and HER. This article provides an overview of C-MFCs for multifunctional catalysis, covering their structure design and synthesis and multifunctional catalysis mechanism and potential applications in clean energy conversion and storage, chemical and energy conversion, and environmental protection. Current challenges and future opportunities in this emerging but rapidly developing field are also discussed.
引用
收藏
页数：21
相关论文
共 50 条
  • [21] Carbon-Based Metal-Free Catalysts for Electrocatalysis beyond the ORR
    Hu, Chuangang
    Dai, Liming
    ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2016, 55 (39) : 11736 - 11758
  • [22] Metal-free, carbon-based catalysts for oxygen reduction reactions
    Zhiyi Wu
    Zafar Iqbal
    Xianqin Wang
    Frontiers of Chemical Science and Engineering, 2015, 9 (03) : 280 - 294
  • [23] Metal-free, carbon-based catalysts for oxygen reduction reactions
    Wu, Zhiyi
    Iqbal, Zafar
    Wang, Xianqin
    FRONTIERS OF CHEMICAL SCIENCE AND ENGINEERING, 2015, 9 (03) : 280 - 294
  • [24] Carbon-Based Metal-Free Electrocatalysis for Energy Conversion, Energy Storage, and Environmental Protection (vol 1, pg 84, 2018)
    Hu, Chuangang
    Xiao, Ying
    Zou, Yuqin
    Dai, Liming
    ELECTROCHEMICAL ENERGY REVIEWS, 2018, 1 (02) : 238 - 238
  • [25] Metal-free, carbon-based materials as catalysts for PEM fuel cells
    Wu, Zhiyi
    Benchafia, Mostafa
    Iqbal, Zafar
    Wang, Xianqin
    ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 2015, 250
  • [26] Polymer-Based Synthetic Routes to Carbon-Based Metal-Free Catalysts
    Gottlieb, Eric
    Matyjaszewski, Krzysztof
    Kowalewski, Tomasz
    ADVANCED MATERIALS, 2019, 31 (13)
  • [27] Carbon-based metal-free electrocatalysts: from oxygen reduction to multifunctional electrocatalysis
    Hu, Chuangang
    Paul, Rajib
    Dai, Quanbin
    Dai, Liming
    CHEMICAL SOCIETY REVIEWS, 2021, 50 (21) : 11785 - +
  • [28] From Carbon-Based Nanotubes to Nanocages for Advanced Energy Conversion and Storage
    Wu, Qiang
    Yang, Lijun
    Wang, Xizhang
    Hu, Zheng
    ACCOUNTS OF CHEMICAL RESEARCH, 2017, 50 (02) : 435 - 444
  • [29] Carbon-Based Nanocages: A New Platform for Advanced Energy Storage and Conversion
    Wu, Qiang
    Yang, Lijun
    Wang, Xizhang
    Hu, Zheng
    ADVANCED MATERIALS, 2020, 32 (27)
  • [30] From carbon-based nanotubes to nanocages for advanced energy conversion and storage
    Hu, Zheng
    ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 2018, 256
12345