The Improvement of Photocatalysis H2 Evolution Over g-C3N4 With Na and Cyano-Group Co-modification

被引:33
|
作者
Liu, Gang [1 ]
Yan, Song [1 ]
Shi, Lei [1 ]
Yao, Lizhu [1 ]
机构
[1] Liaoning Shihua Univ, Coll Chem Chem Engn & Environm Engn, Fushun, Peoples R China
来源
FRONTIERS IN CHEMISTRY | 2019年 / 7卷
关键词
graphitic carbon nitride; Na and cyano-group co-modification; photocatalysis; H-2; evolution; sustainable; GRAPHITIC CARBON NITRIDE; NITROGEN-VACANCY; DOPED G-C3N4; WATER; DEGRADATION; SEMICONDUCTORS; SURFACE; SITES; FUELS;
D O I
10.3389/fchem.2019.00639
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Na and cyano-group co-modified g-C3N4 was easily synthesized and its physicochemical property was completely analyzed. The results manifested that Na and cyano-group modification could heighten visible light absorbed ability and accelerate photoinduced charge separation. When resultant Na and cyano-group co-modified g-C3N4 was splitting water H-2 evolution, its H-2 evolution rate was obviously improved. Furthermore, it also kept excellent stable capacity of H-2 evolution and stability of chemical structure. Hence, this present study does not only develop an efficient strategy to boost photocatalytic property of g-C3N4 based catalysts, but also provides useful guidance for designing more effective photocatalysts.
引用
收藏
页数:7
相关论文
共 50 条
  • [31] Understanding the roles of carbon in carbon/g-C3N4 based photocatalysts for H2 evolution
    Mu Xiao
    Yalong Jiao
    Bin Luo
    Songcan Wang
    Peng Chen
    Miaoqiang Lyu
    Aijun Du
    Lianzhou Wang
    Nano Research, 2023, 16 : 4539 - 4545
  • [32] Recent advances over the doped g-C3N4 in photocatalysis: A review
    Khan, Muhammad Asim
    Mutahir, Sadaf
    Shaheen, Imrana
    Qunhui, Yuan
    Bououdina, Mohamed
    Humayun, Muhammad
    COORDINATION CHEMISTRY REVIEWS, 2025, 522
  • [33] n/n junctioned g-C3N4 for enhanced photocatalytic H2 generation
    Zhou, Minjie
    Hou, Zhaohui
    Zhang, Li
    Liu, Yan
    Gao, Qiongzhi
    Chen, Xiaobo
    SUSTAINABLE ENERGY & FUELS, 2017, 1 (02): : 317 - 323
  • [34] Preparation of C-doped g-C3N4 by Co-polycondensation of melamine and sucrose for improved photocatalytic H2 evolution
    Hussain, Syed Aamir
    Hu, Jun
    Liu, Hongyin
    Aslam, Fawad
    Khan, Salman
    Khan, Luqman
    Jiao, Feipeng
    INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2024, 87 : 705 - 712
  • [35] Photocatalytic H2 evolution and CO2 reduction over phosphorus-doped g-C3N4 nanostructures: Electronic, Optical, and Surface properties
    Mahvelati-Shamsabadi, Tahereh
    Lee, Byeong-Kyu
    RENEWABLE & SUSTAINABLE ENERGY REVIEWS, 2020, 130
  • [36] Construction of Cu7.2S4/g-C3N4 photocatalyst for efficient NIR photocatalysis of H2 production
    Yu, Rui
    Luo, Bifu
    Chen, Min
    Xu, Dongbo
    Wu, Xiaojie
    Li, Di
    Huang, Yuanyong
    Xie, Zhongkai
    Shen, Nanjun
    Meng, Suci
    Shi, Weidong
    INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2023, 48 (63) : 24285 - 24294
  • [37] Preparation of porous C doped g-C3N4 nanosheets controlled by acetamide for photocatalytic H2 evolution
    Wang, Qiongqiong
    Tian, Yaxi
    Chen, Mengyun
    Guan, Rongfeng
    Yuan, Haibin
    INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2022, 47 (71) : 30517 - 30529
  • [38] Expanding g-C3N4 capabilities for photocatalytic H2 production by modification with Ti3C2Tx MXene
    Potapenko, Kseniya O.
    Vasilchenko, Danila B.
    Kurenkova, Anna Yu.
    Saraev, Andrey A.
    Mishchenko, Denis D.
    Gerasimov, Evgeny Yu.
    Kozlova, Ekaterina A.
    INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2025, 99 : 291 - 300
  • [39] Phosphorus and sulphur co-doping of g-C3N4 nanotubes with tunable architectures for superior photocatalytic H2 evolution
    Liu, Zhiguo
    Zhang, Xiao
    Jiang, Zhixiang
    Chen, Hsueh-Shih
    Yang, Ping
    INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2019, 44 (36) : 20042 - 20055
  • [40] The facile synthesis of mesoporous g-C3N4 with highly enhanced photocatalytic H2 evolution performance
    He, Fang
    Chen, Gang
    Zhou, Yansong
    Yu, Yaoguang
    Zheng, Yi
    Hao, Sue
    CHEMICAL COMMUNICATIONS, 2015, 51 (90) : 16244 - 16246