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The Improvement of Photocatalysis H2 Evolution Over g-C3N4 With Na and Cyano-Group Co-modification
被引:33
|作者:
Liu, Gang
[1
]
Yan, Song
[1
]
Shi, Lei
[1
]
Yao, Lizhu
[1
]
机构:
[1] Liaoning Shihua Univ, Coll Chem Chem Engn & Environm Engn, Fushun, Peoples R China
来源:
关键词:
graphitic carbon nitride;
Na and cyano-group co-modification;
photocatalysis;
H-2;
evolution;
sustainable;
GRAPHITIC CARBON NITRIDE;
NITROGEN-VACANCY;
DOPED G-C3N4;
WATER;
DEGRADATION;
SEMICONDUCTORS;
SURFACE;
SITES;
FUELS;
D O I:
10.3389/fchem.2019.00639
中图分类号:
O6 [化学];
学科分类号:
0703 ;
摘要:
Na and cyano-group co-modified g-C3N4 was easily synthesized and its physicochemical property was completely analyzed. The results manifested that Na and cyano-group modification could heighten visible light absorbed ability and accelerate photoinduced charge separation. When resultant Na and cyano-group co-modified g-C3N4 was splitting water H-2 evolution, its H-2 evolution rate was obviously improved. Furthermore, it also kept excellent stable capacity of H-2 evolution and stability of chemical structure. Hence, this present study does not only develop an efficient strategy to boost photocatalytic property of g-C3N4 based catalysts, but also provides useful guidance for designing more effective photocatalysts.
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页数:7
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