Excited states of the negatively charged nitrogen-vacancy color center in diamond

被引：108
|
作者：
Ma, Yuchen [1 ]
Rohlfing, Michael [1 ]
Gali, Adam [2 ]
机构：
[1] Univ Osnabruck, Fachbereich Phys, D-49069 Osnabruck, Germany
[2] Budapest Univ Technol & Econ, Dept Atom Phys, H-1111 Budapest, Hungary
来源：
PHYSICAL REVIEW B | 2010年 / 81卷 / 04期
关键词：
NUCLEAR-SPIN QUBITS; ELECTRONIC-STRUCTURE; COHERENT DYNAMICS; EXCITATIONS; DEFECT; BAND;
D O I：
10.1103/PhysRevB.81.041204
中图分类号：
T [工业技术];
学科分类号：
08 ;
摘要：
Excited states of the negatively charged nitrogen-vacancy color center in diamond are studied using ab initio many-body perturbation theory (within GW approximation and Bethe-Salpeter equation), including electronic exchange, correlation, and electron-hole interaction effects. We find that three singlets, one of which exhibits an intersystem crossing with the excited triplet, may be relevant for the fluorescence process in a way which has never been considered before. The calculated zero-phonon line for the visible excitation and that for the transition among the singlets are in good agreement with the experiments.
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页数：4
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