Temporal trends and spatial variation characteristics of primary air pollutants emissions from coal-fired industrial boilers in Beijing, China

被引:79
|
作者
Xue, Yifeng [1 ,2 ]
Tian, Hezhong [1 ,3 ]
Yan, Jing [2 ]
Zhou, Zhen [2 ]
Wang, Junling [2 ]
Nie, Lei [2 ]
Pan, Tao [2 ,4 ]
Zhou, Junrui [1 ,5 ]
Hua, Shenbing [1 ,3 ]
Wang, Yong [1 ,3 ]
Wu, Xiaoqing [2 ]
机构
[1] Beijing Normal Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100875, Peoples R China
[2] Beijing Municipal Res Inst Environm Protect, Natl Engn Res Ctr Urban Environm Pollut Control, Beijing 100037, Peoples R China
[3] Beijing Normal Univ, Ctr Atmospher Environm Studies, Beijing 100875, Peoples R China
[4] Tianjin Univ, Sch Environm Sci & Technol, Tianjin 300072, Peoples R China
[5] Wuhan Environm Protect Sci Res Inst, Wuhan 43005, Peoples R China
基金
中国国家自然科学基金;
关键词
Coal-fired industrial boilers; Hazardous air pollutants; Emission inventory; Temporal trends; Spatial variation; Substitution of coal with gas; HEBEI BTH REGION; ATMOSPHERIC EMISSIONS; SOURCE APPORTIONMENT; HIGH-RESOLUTION; ORGANIC AEROSOLS; POWER-PLANTS; COMBUSTION; INVENTORY; PM2.5; HYDROCARBONS;
D O I
10.1016/j.envpol.2016.03.047
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Coal-fired combustion is recognized as a significant anthropogenic source of atmospheric compounds in Beijing, causing heavy air pollution events and associated deterioration in visibility. Obtaining an accurate understanding of the temporal trends and spatial variation characteristics of emissions from coal-fired industrial combustion is essential for predicting air quality changes and evaluating the effectiveness of current control measures. In this study, an integrated emission inventory of primary air pollutants emitted from coal-fired industrial boilers in Beijing is developed for the period of 2007-2013 using a technology-based approach. Future emission trends are projected through 2030 based on current energy-related and emission control policies. Our analysis shows that there is a general downward trend in primary air pollutants emissions because of the implementation of stricter local emission standards and the promotion by the Beijing municipal government of converting from coal-fired industrial boilers to gas-fired boilers. However, the ratio of coal consumed by industrial boilers to total coal consumption has been increasing, raising concerns about the further improvement of air quality in Beijing. Our estimates indicate that the total emissions of PM10, PM2.5, SO2, NOx, CO and VOCs from coal-fired industrial boilers in Beijing in 2013 are approximately 19,242 t, 13,345 t, 26,615 t, 22,965 t, 63,779 t and 1406 t, respectively. Under the current environmental policies and relevant energy savings and emission control plans, it may be possible to reduce NOx and other air pollutant emissions by 94% and 90% by 2030, respectively, if advanced flue gas purification technologies are implemented and coal is replaced with natural gas in the majority of existing boilers. (C) 2016 Elsevier Ltd. All rights reserved.
引用
收藏
页码:717 / 726
页数:10
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