Interactions of Water with Mineral Dust Aerosol: Water Adsorption, Hygroscopicity, Cloud Condensation, and Ice Nucleation

被引：303
|
作者：
Tang, Mingjin [1 ]
Cziczo, Daniel J. [2 ,3 ]
Grassian, Vicki H. [1 ,4 ,5 ,6 ,7 ]
机构：
[1] Univ Iowa, Dept Chem, Iowa City, IA 52242 USA
[2] MIT, Dept Earth Atmospher & Planetary Sci, Cambridge, MA 02139 USA
[3] MIT, Civil & Environm Engn, 77 Massachusetts Ave, Cambridge, MA 02139 USA
[4] Univ Calif San Diego, Dept Chem, La Jolla, CA 92093 USA
[5] Univ Calif San Diego, Dept Biochem, La Jolla, CA 92093 USA
[6] Univ Calif San Diego, Dept Nanoengn, La Jolla, CA 92093 USA
[7] Univ Calif San Diego, Scripps Inst Oceanog, La Jolla, CA 92093 USA
来源：
CHEMICAL REVIEWS | 2016年 / 116卷 / 07期
关键词：
GASEOUS-HYDROGEN PEROXIDE; LONG-RANGE TRANSPORT; IN-SITU MEASUREMENTS; HETEROGENEOUS CHEMICAL-KINETICS; ALUMINOSILICATE CLAY-MINERALS; PHASE DIFFUSION-COEFFICIENTS; RELATIVE-HUMIDITY DEPENDENCE; DROPLET ACTIVATION KINETICS; GAS-PARTICLE INTERACTIONS; TITANIUM-DIOXIDE AEROSOL;
D O I：
10.1021/acs.chemrev.5b00529
中图分类号：
O6 [化学];
学科分类号：
0703 ;
摘要：
Mineral dust aerosol is one of the major types of aerosol present in the troposphere. The molecular level interactions of water vapor with mineral dust are of global significance. Hygroscopicity, light scattering and absorption, heterogneous reactivity and the ability to form clouds are'all related to water-dust interactions. In this review article, experimental techniques to probe water interactions with dust and theoretical frameworks to understand these interactions are discussed. A comprehensive overview of laboratory studies of water adsorption, hygroscopicity, cloud condensation, and ice nucleation of fresh and atmspherically aged mineral dust particles is provided. Finally, we relate laboratory studies and theoretical simulations that provide fundemental insights into these processes on the molecular level with field measurements that illustrate the atmospheric significance of these processes. Overall, the details of water interactions with mineral dust are covered from multiple perspectives in this review article.
引用
收藏
页码：4205 / 4259
页数：55
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