Double-Cable Conjugated Polymers with Fullerene Pendant for Single-Component Organic Solar Cells

被引：15
|
作者：
Liu, Bai-Qiao [1 ]
Xu, Yun-Hua [1 ]
Liu, Feng [4 ]
Xie, Cheng-Cheng [2 ,3 ]
Liang, Shi-Jie [2 ,3 ]
Chen, Qiao-Mei [2 ,3 ]
Li, Wei-Wei [2 ,3 ]
机构：
[1] Beijing Jiaotong Univ, Sch Sci, Dept Chem, Beijing 100044, Peoples R China
[2] Beijing Univ Chem Technol, Beijing Adv Innovat Ctr Soft Matter Sci & Engn, Beijing 100029, Peoples R China
[3] Beijing Univ Chem Technol, State Key Lab Organ Inorgan Composites, Beijing 100029, Peoples R China
[4] Hebei Univ, Coll Basic Med, Baoding 071002, Peoples R China
来源：
CHINESE JOURNAL OF POLYMER SCIENCE | 2022年 / 40卷 / 08期
基金：
北京市自然科学基金; 中国国家自然科学基金;
关键词：
Double-cable conjugated polymers; Single-component organic solar cells; Fullerene; Donor-acceptor" conjugated polymers; Microphase separation; ACCEPTOR BLOCK-COPOLYMERS; PHOTOVOLTAIC PROPERTIES; MICROPHASE SEPARATION; POLYTHIOPHENE; ENABLES; DONORS;
D O I：
10.1007/s10118-022-2732-2
中图分类号：
O63 [高分子化学（高聚物）];
学科分类号：
070305 ; 080501 ; 081704 ;
摘要：
In this work, the "functionalization-polymerization" (FP) method has been used to construct fullerene-contained double-cable conjugated polymers with "donor-acceptor" backbones. It was realized via synthesizing a fullerene-contained monomer and performing Stille polymerization. With this method, a series of double-cable conjugated polymers with different fullerene contents were developed and applied into single-component organic solar cells. The power conversion efficiencies (PCEs) based on these polymers increased from 0.71% to 1.71% with the enhanced fullerene contents. The relatively low PCEs might be originated from the poor microstructure in these polymers. These new conjugated polymers with molecular heterojunction would show potential application in organic electronic devices.
引用
收藏
页码：898 / 904
页数：7
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