Mobile source contributions to ambient ozone and particulate matter in 2025

被引:31
|
作者
Zawacki, Margaret [1 ]
Baker, Kirk R. [2 ]
Phillips, Sharon [2 ]
Davidson, Kenneth [3 ]
Wolfe, Philip [4 ]
机构
[1] US EPA, Off Transportat & Air Qual, 2000 Traverwood Dr, Ann Arbor, MI 48105 USA
[2] US EPA, Off Air Qual Planning & Stand, Res Triangle Pk, NC 27711 USA
[3] US EPA, Off Transportat & Air Qual, San Francisco, CA USA
[4] US EPA, Ann Arbor, MI 48105 USA
关键词
Mobile source; Source apportionment; Air pollution; Ozone; Particulate matter; PRINCIPAL COMPONENT ANALYSIS; AIR-POLLUTION; SOURCE APPORTIONMENT; EMISSION INVENTORY; UNITED-STATES; MODEL; NOX; CALIFORNIA; IMPACTS; EASTERN;
D O I
10.1016/j.atmosenv.2018.04.057
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The contribution of precursor emissions from 17 mobile source sectors to ambient ozone and fine particulate matter levels across the U.S. were evaluated, using the CAMx photochemical model, to identify which mobile source sectors are projected to have the largest impacts on air pollution in 2025. Both onroad and nonroad sectors contribute considerably to projected air pollution across much of the country. Summer ozone season ozone contributions between 2 and 5 ppb, which are among the highest levels presented on the maps of mobile source sectors, are largely found in the southeast United States from the onroad sectors, most notably light-duty and heavy-duty vehicles, and along the coastline from the Category 3 (C3) marine sector. Annual average PM2.5 contributions between 0.5 and 0.9 mu g/m(3), which are among the highest levels presented on the maps of mobile source sectors, are found throughout the Midwest and along portions of the east and west coast from onroad sectors as well as nonroad diesel and rail sectors. Additionally, contributions of precursor emissions to ambient ozone and PM2.5 levels were evaluated to understand the range of impacts from precursors in the various mobile source sectors. For most mobile source sectors, in most locations, NOx emissions contributed more to ozone than VOC emissions, and secondary PM2.5 contributed more to ambient PM2.5 than primary PM2.5. The largest ozone levels on the maps showing contributions from mobile source NOx emissions tended to be between 2 and 5 ppb, while the largest ozone levels on the maps showing contributions from mobile source VOC emissions tended to be between 0.9 and 2 ppb, except for southern California where ozone contributions from VOC emissions from onroad light duty vehicles were between 2 and 5 ppb. The largest contributions to ambient PM2.5 on the maps showing primary and secondary contributions from mobile source sectors tended to be between 0.1 and 0.5 mu g/m(3). The contribution from primary PM2.5 extended over localized areas (urban-scale) and the contribution from secondary PM2.5 extended over more regional (multi-state) areas.
引用
收藏
页码:129 / 141
页数:13
相关论文
共 50 条
  • [31] Air particulate matter pollution in Ulaanbaatar, Mongolia: determination of composition, source contributions and source locations
    Davy, Perry K.
    Gunchin, Gerelmaa
    Markwitz, Andreas
    Trompetter, William J.
    Barry, Bernard J.
    Shagjjamba, Dagva
    Lodoysamba, Sereeter
    [J]. ATMOSPHERIC POLLUTION RESEARCH, 2011, 2 (02) : 126 - 137
  • [32] Associations between ambient fine particulate matter and child respiratory infection: The role of particulate matter source composition in Dhaka, Bangladesh
    Sherris, Allison R.
    Begum, Bilkis A.
    Baiocchi, Michael
    Goswami, Doli
    Hopke, Philip K.
    Brooks, W. Abdullah
    Luby, Stephen P.
    [J]. ENVIRONMENTAL POLLUTION, 2021, 290
  • [33] Apportionment of ambient primary and secondary fine particulate matter at the Pittsburgh National Energy Laboratory particulate matter characterization site using positive matrix factorization and a potential source contributions function analysis
    Martello, Donald V.
    Pekney, Natalie J.
    Anderson, Richard R.
    Davidson, Cliff I.
    Hopke, Philip K.
    Kim, Eugene
    Christensen, William F.
    Mangelson, Nolan F.
    Eatough, Delbert J.
    [J]. JOURNAL OF THE AIR & WASTE MANAGEMENT ASSOCIATION, 2008, 58 (03) : 357 - 368
  • [34] Study of condensable particulate matter from stationary combustion sources: Source profiles, emissions, and impact on ambient fine particulate matter
    Tong, Huanhuan
    Wang, Yangjun
    Huang, Ling
    Su, Qingfang
    Yi, Xin
    Zhai, Hehe
    Jiang, Sen
    Liu, Hanqing
    Liao, Jiaqiang
    Li, Li
    [J]. SCIENCE OF THE TOTAL ENVIRONMENT, 2024, 954
  • [35] Premature Mortality Attributable to Particulate Matter in China: Source Contributions and Responses to Reductions
    Hu, Jianlin
    Huang, Lin
    Chen, Mindong
    Liao, Hong
    Zhang, Hongliang
    Wang, Shuxiao
    Zhang, Qiang
    Ying, Qi
    [J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2017, 51 (17) : 9950 - 9959
  • [36] Mobile Source and Livestock Feed Contributions to Regional Ozone Formation in Central California
    Hu, Jianlin
    Howard, Cody J.
    Mitloehner, Frank
    Green, Peter G.
    Kleeman, Michael J.
    [J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2012, 46 (05) : 2781 - 2789
  • [37] Source Contributions to Fine Particulate Matter and Attributable Mortality in India and the Surrounding Region
    Chatterjee, Deepangsu
    McDuffie, Erin E.
    Smith, Steven J.
    Bindle, Liam
    Van Donkelaar, Aaron
    Hammer, Melanie S.
    Venkataraman, Chandra
    Brauer, Michael
    Martin, Randall V.
    [J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2023, 57 (28) : 10263 - 10275
  • [38] A QUANTITATIVE ASSESSMENT OF SOURCE CONTRIBUTIONS TO INHALABLE PARTICULATE MATTER POLLUTION IN METROPOLITAN BOSTON
    LOWENTHAL, DH
    RAHN, KA
    [J]. ATMOSPHERIC ENVIRONMENT, 1987, 21 (01) : 257 - 259
  • [39] Saccharide composition in atmospheric particulate matter in the southwest US and estimates of source contributions
    Jia, Yuling
    Clements, Andrea L.
    Fraser, Matthew P.
    [J]. JOURNAL OF AEROSOL SCIENCE, 2010, 41 (01) : 62 - 73
  • [40] A QUANTITATIVE ASSESSMENT OF SOURCE CONTRIBUTIONS TO INHALABLE PARTICULATE MATTER POLLUTION IN METROPOLITAN BOSTON
    THURSTON, GD
    SPENGLER, JD
    [J]. ATMOSPHERIC ENVIRONMENT, 1985, 19 (01) : 9 - 25