Using a combination of local and global magnetometry, dimensional analysis and numerical simulations we investigate the dynamics of magnetic phase cluster formation across the first-order magnetic-field-driven magnetostructural transition in Gd5Ge4 at 6 K, where the transformation is completely irreversible, and at 35 K, where the reversibility is restored due to rising thermal fluctuations. We have previously shown, using scanning Hall probe images, that the transition involves phase separated clusters. Here we discuss these images in the context of a random nucleation and growth model, focusing on the relation between microscopic and macroscopic behaviours. The purpose of the work is to set up a framework for the analysis of these materials and it has implications for future discoveries of related functional magnetic materials where first-order, disorder-broadened transitions dominate key physical properties.
机构:
Wolfson Centre for Magnetics, Cardiff University, Cardiff CF24 3AA, United KingdomWolfson Centre for Magnetics, Cardiff University, Cardiff CF24 3AA, United Kingdom
Hadimani, R.L.
Melikhov, Y.
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Wolfson Centre for Magnetics, Cardiff University, Cardiff CF24 3AA, United KingdomWolfson Centre for Magnetics, Cardiff University, Cardiff CF24 3AA, United Kingdom
Melikhov, Y.
Snyder, J.E.
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Wolfson Centre for Magnetics, Cardiff University, Cardiff CF24 3AA, United KingdomWolfson Centre for Magnetics, Cardiff University, Cardiff CF24 3AA, United Kingdom
Snyder, J.E.
Jiles, D.C.
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Wolfson Centre for Magnetics, Cardiff University, Cardiff CF24 3AA, United KingdomWolfson Centre for Magnetics, Cardiff University, Cardiff CF24 3AA, United Kingdom
机构:
Los Alamos Natl Lab, Div Theoret, T-4, Los Alamos, NM 87545 USA
Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USALos Alamos Natl Lab, Div Theoret, T-4, Los Alamos, NM 87545 USA
Zhu, W.
Sheng, D. N.
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机构:
Calif State Univ Northridge, Dept Phys, Northridge, CA 91325 USALos Alamos Natl Lab, Div Theoret, T-4, Los Alamos, NM 87545 USA
Sheng, D. N.
Zhu, Jian-Xin
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Los Alamos Natl Lab, Div Theoret, T-4, Los Alamos, NM 87545 USA
Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USALos Alamos Natl Lab, Div Theoret, T-4, Los Alamos, NM 87545 USA
机构:
US DOE, Div Mat Sci & Engn, Ames Lab, Ames, IA 50011 USA
Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USAUS DOE, Div Mat Sci & Engn, Ames Lab, Ames, IA 50011 USA
机构:
Iowa State Univ, Mat & Engn Phys Program, Ames Lab, US DOE, Ames, IA 50011 USAIowa State Univ, Mat & Engn Phys Program, Ames Lab, US DOE, Ames, IA 50011 USA
Mudryk, Y
Holm, AP
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机构:Iowa State Univ, Mat & Engn Phys Program, Ames Lab, US DOE, Ames, IA 50011 USA
Holm, AP
Gschneidner, KA
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机构:Iowa State Univ, Mat & Engn Phys Program, Ames Lab, US DOE, Ames, IA 50011 USA
Gschneidner, KA
Pecharsky, VK
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机构:Iowa State Univ, Mat & Engn Phys Program, Ames Lab, US DOE, Ames, IA 50011 USA