In situ diffusion experiment in granite: Phase I

被引:44
|
作者
Vilks, P [1 ]
Cramer, JJ
Jensen, M
Miller, NH
Miller, HG
Stanchell, FW
机构
[1] Atom Energy Canada Ltd, Whiteshell Labs, Pinawa, MB R0E 1L0, Canada
[2] Ontario Power Generat, Nucl Waste Management Div, Toronto, ON M5G 1X6, Canada
关键词
diffusion; in situ; experiment; granite; iodide;
D O I
10.1016/S0169-7722(02)00135-3
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
A program of in situ experiments, supported by laboratory studies, was initiated to study diffusion in sparsely fractured rock (SFR), with a goal of developing an understanding of diffusion processes within intact crystalline rock. Phase I of the in situ diffusion experiment was started in 1996, with the purpose of developing a methodology for estimating diffusion parameter values. Four in situ diffusion experiments, using a conservative iodide tracer, were performed in highly stressed SFR at a depth of 450 m in the Underground Research Laboratory (URL). The experiments, performed over a 2 year period, yielded rock permeability estimates of 2 x 10(-21) m(2) and effective diffusion coefficients varying from 2.1 x 10(-14) to 1.9 x 10(-13) m(2)/s, which were estimated using the MOTIF code. The in situ diffusion profiles reveal a characteristic "dog leg" pattern, with iodide concentrations decreasing rapidly within a centimeter of the open borehole wall. It is hypothesized that this is an artifact of local stress redistribution and creation of a zone of increased constrictivity close to the borehole wall. A comparison of estimated in situ and laboratory diffasivities and permeabilities provides evidence that the physical properties of rock samples removed from high-stress regimes change. As a result of the lessons learnt during Phase I, a Phase II in situ program has been initiated to improve our general understanding of diffusion in SFR. Crown Copyright (C) 2002 Published by Elsevier Science B.V. All rights reserved.
引用
收藏
页码:191 / 202
页数:12
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