Air quality;
Co-pollution;
Six criteria pollutants;
Health risk;
SHORT-TERM EXPOSURE;
OZONE POLLUTION;
SURFACE OZONE;
QUALITY;
COMPLEX;
INDEX;
MULTIPOLLUTANT;
IMPACTS;
CITIES;
NORTH;
D O I:
10.1016/j.atmosenv.2021.118829
中图分类号:
X [环境科学、安全科学];
学科分类号:
08 ;
0830 ;
摘要:
We characterized air pollution over China during 2014-2020, with a novel focus on multi-pollutant air pollution (MPAP) for the first time (defined as co-pollution of two or more contaminants) which was quite common in China but has not been evaluated, and assessed associated health risks of air pollution exposure which specially took into account the effects of exposure to multi-pollutant mixture, by introducing a health-risk based and multi-pollutant air quality index (HAQI). High values of MPAP days were mostly distributed over North China with a 7-year average of 51.9 MPAP days. The severest MPAP occurred in winter with PM2.5-PM10 co-pollution accounting for 80-100% of MPAP days for six provinces of North China. One interesting phenomenon was that MPAP days exhibited almost overall declines (average trend of -11.9 days yr(-1)) over North China during 2014-2020 due to decreases in PM2.5-PM10 and PM2.5-O-3 co-pollution days, while single-pollutant air pollution (SPAP) days showed almost overall rising trends with an average trend of +8.0 days yr(-1) which was attributed to rapid increases in O-3 pollution days. The HAQI also exhibited high values over North China with a 7-year average HAQI value of 102.4. Health risks were the greatest in winter with 89.4% of population exposed to "unhealthy " air (HAQI > 100) and 20.1% of population suffering from "very unhealthy " (HAQI > 200) air over North China. Thanks to the mitigation of particulate pollution (shown as decreases in PM2.5 pollution days, PM2.5-PM10 co-pollution days, and PM2.5-O-3 co-pollution days), health risks in five provinces of North China except Shanxi experienced remarkable declines with HAQI trends of-3.1 yr(-1) -9.7 yr(-1) during 2014-2020. Unrelieved particulate pollution and deteriorating O-3 pollution, however, jointly led to rising health risks for Shanxi. These findings are expected to provide a scientific cognition of complex air pollution and associated health impacts.
机构:
Hong Kong Polytech Univ, Dept Civil & Environm Engn, Hong Kong 999077, Peoples R ChinaHong Kong Polytech Univ, Dept Civil & Environm Engn, Hong Kong 999077, Peoples R China
Liu, Yiming
Wang, Tao
论文数: 0引用数: 0
h-index: 0
机构:
Hong Kong Polytech Univ, Dept Civil & Environm Engn, Hong Kong 999077, Peoples R ChinaHong Kong Polytech Univ, Dept Civil & Environm Engn, Hong Kong 999077, Peoples R China
机构:
Environm Canada, Atmospher Sci & Technol Directorate, Air Qual Res Div, Toronto, ON M3H 5T4, CanadaEnvironm Canada, Atmospher Sci & Technol Directorate, Air Qual Res Div, Toronto, ON M3H 5T4, Canada
Brook, Jeffrey R.
Demerjian, Kenneth L.
论文数: 0引用数: 0
h-index: 0
机构:
SUNY Albany, Atmospher Sci Res Ctr, Albany, NY 12203 USA
SUNY Albany, Dept Earth & Atmospher Sci, Albany, NY 12203 USAEnvironm Canada, Atmospher Sci & Technol Directorate, Air Qual Res Div, Toronto, ON M3H 5T4, Canada
Demerjian, Kenneth L.
Hidy, George
论文数: 0引用数: 0
h-index: 0
机构:
Envair Aerochem, Placitas, NM 87043 USAEnvironm Canada, Atmospher Sci & Technol Directorate, Air Qual Res Div, Toronto, ON M3H 5T4, Canada
Hidy, George
Molina, Luisa T.
论文数: 0引用数: 0
h-index: 0
机构:
MIT, La Jolla, CA 92037 USA
Molina Ctr Energy & Environm, La Jolla, CA 92037 USAEnvironm Canada, Atmospher Sci & Technol Directorate, Air Qual Res Div, Toronto, ON M3H 5T4, Canada
Molina, Luisa T.
Pennell, William I.
论文数: 0引用数: 0
h-index: 0
机构:
Columbia Res & Educ Associates, Columbia, WA 99301 USAEnvironm Canada, Atmospher Sci & Technol Directorate, Air Qual Res Div, Toronto, ON M3H 5T4, Canada
Pennell, William I.
Scheffe, Richard
论文数: 0引用数: 0
h-index: 0
机构:
US EPA, Durham, NC 27711 USAEnvironm Canada, Atmospher Sci & Technol Directorate, Air Qual Res Div, Toronto, ON M3H 5T4, Canada
机构:
Univ Hong Kong, Dept Elect & Elect Engn, Hong Kong, Peoples R ChinaUniv Hong Kong, Dept Elect & Elect Engn, Hong Kong, Peoples R China
Maji, Kamal Jyoti
Li, Victor O. K.
论文数: 0引用数: 0
h-index: 0
机构:
Univ Hong Kong, Dept Elect & Elect Engn, Hong Kong, Peoples R ChinaUniv Hong Kong, Dept Elect & Elect Engn, Hong Kong, Peoples R China
Li, Victor O. K.
Lam, Jacqueline C. K.
论文数: 0引用数: 0
h-index: 0
机构:
Univ Hong Kong, Dept Elect & Elect Engn, Hong Kong, Peoples R China
Univ Cambridge, Judge Business Sch, Energy Policy Res Grp, Hong Kong, Peoples R China
Univ Cambridge, Dept Comp Sci & Technol, Hong Kong, Peoples R China
MIT, MIT Energy Initiat, CEEPR, Hong Kong, Peoples R ChinaUniv Hong Kong, Dept Elect & Elect Engn, Hong Kong, Peoples R China
机构:
Univ London London Sch Econ & Polit Sci, Dept Govt, London WC2A 2AE, EnglandMIT, Joint Program Sci & Policy Global Change, Cambridge, MA 02139 USA
Matus, Kira
Nam, Kyung-Min
论文数: 0引用数: 0
h-index: 0
机构:
MIT, Joint Program Sci & Policy Global Change, Cambridge, MA 02139 USAMIT, Joint Program Sci & Policy Global Change, Cambridge, MA 02139 USA
Nam, Kyung-Min
Selin, Noelle E.
论文数: 0引用数: 0
h-index: 0
机构:
MIT, Engn Syst Div, Cambridge, MA 02139 USA
MIT, Dept Earth Atmospher & Planetary Sci, Cambridge, MA 02139 USAMIT, Joint Program Sci & Policy Global Change, Cambridge, MA 02139 USA
Selin, Noelle E.
Lamsal, Lok N.
论文数: 0引用数: 0
h-index: 0
机构:
Dalhousie Univ, Dept Phys & Atmospher Sci, Halifax, NS B3H 4R2, CanadaMIT, Joint Program Sci & Policy Global Change, Cambridge, MA 02139 USA
Lamsal, Lok N.
Reilly, John M.
论文数: 0引用数: 0
h-index: 0
机构:
MIT, Joint Program Sci & Policy Global Change, Cambridge, MA 02139 USAMIT, Joint Program Sci & Policy Global Change, Cambridge, MA 02139 USA
Reilly, John M.
Paltsev, Sergey
论文数: 0引用数: 0
h-index: 0
机构:
MIT, Joint Program Sci & Policy Global Change, Cambridge, MA 02139 USAMIT, Joint Program Sci & Policy Global Change, Cambridge, MA 02139 USA
Paltsev, Sergey
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GLOBAL ENVIRONMENTAL CHANGE-HUMAN AND POLICY DIMENSIONS,
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机构:
Univ Stuttgart, Inst Energy Econ & Rat Use Energy, D-70565 Stuttgart, GermanyUniv Stuttgart, Inst Energy Econ & Rat Use Energy, D-70565 Stuttgart, Germany
Reis, S
Nitter, S
论文数: 0引用数: 0
h-index: 0
机构:
Univ Stuttgart, Inst Energy Econ & Rat Use Energy, D-70565 Stuttgart, GermanyUniv Stuttgart, Inst Energy Econ & Rat Use Energy, D-70565 Stuttgart, Germany
Nitter, S
Friedrich, R
论文数: 0引用数: 0
h-index: 0
机构:
Univ Stuttgart, Inst Energy Econ & Rat Use Energy, D-70565 Stuttgart, GermanyUniv Stuttgart, Inst Energy Econ & Rat Use Energy, D-70565 Stuttgart, Germany