Pressure-Induced Argon Insertion into an Auxetic Small Pore Zeolite

被引：26
|
作者：
Lee, Yongjae [3 ]
Hriljac, Joseph A. [4 ]
Vogt, Thomas [1 ,2 ]
机构：
[1] Univ S Carolina, NanoCtr, Columbia, SC 29208 USA
[2] Univ S Carolina, Dept Chem & Biochem, Columbia, SC 29208 USA
[3] Yonsei Univ, Dept Earth Syst Sci, Seoul 120749, South Korea
[4] Univ Birmingham, Sch Chem, Birmingham B15 2TT, W Midlands, England
来源：
JOURNAL OF PHYSICAL CHEMISTRY C | 2010年 / 114卷 / 15期
关键词：
NOBLE-GAS SOLUBILITIES; SILICATE MELTS; NEUTRON-DIFFRACTION; CRYSTAL-STRUCTURES; LAUMONTITE; BEHAVIOR; NATROLITE; XENON; DISTORTION; FRAMEWORK;
D O I：
10.1021/jp911231p
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
We report that natrolite,Na16Al16Si24O48 center dot 16H(2)O, a small pore auxetic zeolite can incorporate significant amounts of Argon under moderate pressure- and temperature conditions resulting in Na16Al16Si24O80 center dot 16H(2)O center dot 6Ar. This material has a similar to 6.5% larger unit cell than natrolite at ambient conditions and its structure is related to Na16Al16Si24O80 center dot 24H(2)O, an intermediate superhydrated natrolite referred to as para-natrolite. Argon insertion under pressure into auxetic frameworks such as natrolites is an important and overlooked confinement mechanism with potential applications and implications.
引用
收藏
页码：6922 / 6927
页数：6
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